Three-dimensional, two-phase, CFD model for the design of a direct methanol fuel cell

被引:38
作者
Danilov, Valeri A.
Lim, Jongkoo
Moon, Il
Chang, Hyuk
机构
[1] Yonsei Univ, Dept Chem Engn, Seoul 120749, South Korea
[2] Samsung Adv Inst Technol, Suwon 400600, South Korea
关键词
direct methanol fuel cell; two-phase model; gas management; flow-field design; computational fluid dynamics; PROTON-EXCHANGE MEMBRANE; NUMERICAL-SIMULATION; GAS EVOLUTION; MASS-TRANSFER; FLOW;
D O I
10.1016/j.jpowsour.2006.07.071
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
This study presents a computational fluid dynamics.(CFD) model for modelling gas evolution and current distribution in a direct methanol fuel cell (DMFC). The improved two-phase model includes a new sub-model for estimating the interface mass transfer without empirical correlations. Simulation results in a horizontal channel of the DMFC agree with typical trends reported in the literature for bubbly flows. The increase in inlet flow rate is found to lead to a decrease in the gas content in the outlet of the anode channels. A case study illustrates applications of the CFD model for modelling gas evolution and current distribution in a DMFC with a parallel flow-field design. Simulation results with a improved two-phase model provide an explanation of experimental observations of a transparent DMFC with parallel channels. An improved three-dimensional CFD model includes all relevant phenomena and is valuable for gas management in a DMFC design. (c) 2006 Elsevier B.V. All rights reserved.
引用
收藏
页码:992 / 1002
页数:11
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