In situ intercalation strategies for device-quality hybrid inorganic-organic self-assembled quantum wells

被引:44
作者
Pradeesh, K. [1 ]
Baumberg, J. J. [2 ]
Prakash, G. Vijaya [1 ]
机构
[1] Indian Inst Technol, Dept Phys, Nanophoton Lab, New Delhi 110016, India
[2] Univ Cambridge, Nanophoton Ctr, Cavendish Lab, Cambridge CB3 0HE, England
基金
英国工程与自然科学研究理事会;
关键词
excitons; multilayers; organic-inorganic hybrid materials; photoluminescence; quantum well devices; thin films; THIN-FILMS; PEROVSKITE;
D O I
10.1063/1.3186639
中图分类号
O59 [应用物理学];
学科分类号
摘要
Thin films of self-organized quantum wells of inorganic-organic hybrid perovskites of (C6H9C2H4NH3)(2)PbI4 are formed from a simple intercalation strategy to yield well-ordered uniform films over centimeter-size scales. These films compare favorably with traditional solution-chemistry-synthesized thin films. The hybrid films show strong room-temperature exciton-related absorption and photoluminescence, which shift with fabrication protocol. We demonstrate the potential of this method for electronic and photonic device applications.
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页数:3
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共 15 条
[1]   Poly[bis[2-(1-cyclohexenyl)ethylammonium] di-μ-iodo-diodo-plumbate(II)] [J].
Billing, David G. ;
Lemmerer, Andreas .
ACTA CRYSTALLOGRAPHICA SECTION C-STRUCTURAL CHEMISTRY, 2006, 62 (07) :M269-M271
[2]   Patterning and photolumine scent properties of perovskite-type organic/inorganic hybrid luminescent films by soft lithography [J].
Cheng, ZY ;
Wang, Z ;
Xing, RB ;
Han, YC ;
Lin, J .
CHEMICAL PHYSICS LETTERS, 2003, 376 (3-4) :481-486
[3]   Strong exciton-photon coupling in a length tunable optical microcavity with J-aggregate dye heterostructures -: art. no. 041110 [J].
Finlayson, CE ;
Prakash, GV ;
Baumberg, JJ .
APPLIED PHYSICS LETTERS, 2005, 86 (04) :041110-1
[4]   OPTICAL-PROPERTIES DUE TO ELECTRONIC-TRANSITIONS IN 2-DIMENSIONAL SEMICONDUCTORS (CNH2N + 1NH3)2PBI4 [J].
ISHIHARA, T ;
TAKAHASHI, J ;
GOTO, T .
PHYSICAL REVIEW B, 1990, 42 (17) :11099-11107
[5]   EXCITON-STATE IN TWO-DIMENSIONAL PEROVSKITE SEMICONDUCTOR (C10H21NH3)2PBI4 [J].
ISHIHARA, T ;
TAKAHASHI, J ;
GOTO, T .
SOLID STATE COMMUNICATIONS, 1989, 69 (09) :933-936
[6]   Organic-inorganic hybrid materials as semiconducting channels in thin-film field-effect transistors [J].
Kagan, CR ;
Mitzi, DB ;
Dimitrakopoulos, CD .
SCIENCE, 1999, 286 (5441) :945-947
[7]   Fabrication of two-dimensional layered perovskite [NH3(CH2)12NH3]PbX4 thin films using a self-assembly method [J].
Matsui, T ;
Yamaguchi, A ;
Takeoka, Y ;
Rikukawa, M ;
Sanui, K .
CHEMICAL COMMUNICATIONS, 2002, (10) :1094-1095
[8]   CONDUCTING TIN HALIDES WITH A LAYERED ORGANIC-BASED PEROVSKITE STRUCTURE [J].
MITZI, DB ;
FEILD, CA ;
HARRISON, WTA ;
GULOY, AM .
NATURE, 1994, 369 (6480) :467-469
[9]   Thin-film deposition of organic-inorganic hybrid materials [J].
Mitzi, DB .
CHEMISTRY OF MATERIALS, 2001, 13 (10) :3283-3298
[10]   EXCITONS IN SELF-ORGANIZED SEMICONDUCTOR-INSULATOR SUPERLATTICES - PBI-BASED PEROVSKITE COMPOUNDS [J].
MULJAROV, EA ;
TIKHODEEV, SG ;
GIPPIUS, NA ;
ISHIHARA, T .
PHYSICAL REVIEW B, 1995, 51 (20) :14370-14378