Band gap engineering and spatial confinement of optical phonon in ZnO quantum dots

被引:103
作者
Lin, Kuo-Feng
Cheng, Hsin-Ming
Hsu, -Cheng Hsu
Hsieh, Wen-Feng
机构
[1] Natl Chiao Tung Univ, Dept Photon, Inst Electroopt Engn, Hsinchu 30050, Taiwan
[2] Ind Technol Res Inst, Mat & Chem Res Labs, Hsinchu 310, Taiwan
关键词
D O I
10.1063/1.2218775
中图分类号
O59 [应用物理学];
学科分类号
摘要
Both band gap engineering and spatial confinement of optical phonon were observed depending upon the size of ZnO quantum dots at room temperature. Size-dependent blueshifts of photoluminescence and absorption spectra reveal the quantum confinement effect. The measured Raman spectral shift and asymmetry for the E-2(high) mode caused by localization of optical phonons agree well with that calculated by using the modified spatial correlation model. (c) 2006 American Institute of Physics.
引用
收藏
页数:3
相关论文
共 28 条
[21]   Optical phonon confinement in zinc oxide nanoparticles [J].
Rajalakshmi, M ;
Arora, AK ;
Bendre, BS ;
Mahamuni, S .
JOURNAL OF APPLIED PHYSICS, 2000, 87 (05) :2445-2448
[22]   THE ONE PHONON RAMAN-SPECTRUM IN MICROCRYSTALLINE SILICON [J].
RICHTER, H ;
WANG, ZP ;
LEY, L .
SOLID STATE COMMUNICATIONS, 1981, 39 (05) :625-629
[23]   UV RESONANT RAMAN SCATTERING IN ZNO [J].
SCOTT, JF .
PHYSICAL REVIEW B, 1970, 2 (04) :1209-&
[24]   Optical properties of confined polaronic excitons in spherical ionic quantum dots [J].
Senger, RT ;
Bajaj, KK .
PHYSICAL REVIEW B, 2003, 68 (04)
[25]   Multiphonon resonant Raman scattering in ZnO crystals and nanostructured layers [J].
Ursaki, VV ;
Tiginyanu, IM ;
Zalamai, VV ;
Rusu, EV ;
Emelchenko, GA ;
Masalov, VM ;
Samarov, EN .
PHYSICAL REVIEW B, 2004, 70 (15) :155204-1
[26]   Raman study for E2 phonon of ZnO in Zn1-xMnxO nanoparticles -: art. no. 086105 [J].
Wang, JB ;
Zhong, HM ;
Li, ZF ;
Lu, W .
JOURNAL OF APPLIED PHYSICS, 2005, 97 (08)
[27]   Size dependence of electron-phonon coupling in ZnO nanowires [J].
Wang, RP ;
Xu, G ;
Jin, P .
PHYSICAL REVIEW B, 2004, 69 (11)
[28]   Raman spectral study of silicon nanowires: High-order scattering and phonon confinement effects [J].
Wang, RP ;
Zhou, GW ;
Liu, YL ;
Pan, SH ;
Zhang, HZ ;
Yu, DP ;
Zhang, Z .
PHYSICAL REVIEW B, 2000, 61 (24) :16827-16832