Nanoscale design to enable the revolution in renewable energy

被引:340
作者
Baxter, Jason [1 ]
Bian, Zhixi [2 ]
Chen, Gang [3 ]
Danielson, David [4 ]
Dresselhaus, Mildred S. [5 ,6 ]
Fedorov, Andrei G. [7 ,8 ]
Fisher, Timothy S. [10 ]
Jones, Christopher W. [11 ]
Maginn, Edward [12 ]
Kortshagen, Uwe [13 ]
Manthiram, Arumugam [14 ,15 ]
Nozik, Arthur [16 ]
Rolison, Debra R. [17 ]
Sands, Timothy [9 ,18 ]
Shi, Li [14 ,15 ]
Sholl, David [11 ]
Wu, Yiying [19 ]
机构
[1] Drexel Univ, Dept Chem & Biol Engn, Philadelphia, PA 19104 USA
[2] Univ Calif Santa Cruz, Dept Elect Engn, Santa Cruz, CA 95064 USA
[3] MIT, Dept Mech Engn, Cambridge, MA 02139 USA
[4] Gen Catalyst Partners, Cambridge, MA 02139 USA
[5] MIT, Dept Phys, Cambridge, MA 02139 USA
[6] MIT, Dept Elect Engn & Comp Sci, Cambridge, MA 02139 USA
[7] Georgia Inst Technol, George W Woodruff Sch Mech Engn, Atlanta, GA 30332 USA
[8] Petit Inst Bioengn & Biosci, Atlanta, GA 30332 USA
[9] Purdue Univ, Birck Nanotechnol Ctr, Sch Mat Engn, W Lafayette, IN 47907 USA
[10] Purdue Univ, Sch Mech Engn, W Lafayette, IN 47907 USA
[11] Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA
[12] Univ Notre Dame, Dept Chem & Biomol Engn, Notre Dame, IN 46556 USA
[13] Univ Minnesota, Dept Mech Engn, Minneapolis, MN 55455 USA
[14] Univ Texas Austin, Texas Mat Inst, Austin, TX 78712 USA
[15] Univ Texas Austin, Dept Mech Engn, Austin, TX 78712 USA
[16] Ctr Revolutionary Solar Photoconvers, Natl Renewable Energy Lab, Golden, CO 80401 USA
[17] USN, Res Lab, Surface Chem Branch, Washington, DC 20375 USA
[18] Purdue Univ, Sch Elect & Comp Engn, W Lafayette, IN 47907 USA
[19] Ohio State Univ, Dept Chem, Columbus, OH 43210 USA
基金
美国国家科学基金会;
关键词
MULTIPLE EXCITON GENERATION; HYDROGEN-STORAGE; THERMAL-CONDUCTIVITY; ELECTRODE MATERIALS; THERMOELECTRIC PERFORMANCE; PHOTOCATALYTIC ACTIVITY; CONVERSION EFFICIENCY; TRANSPORTATION FUELS; GAMMA-VALEROLACTONE; MESOPOROUS SILICA;
D O I
10.1039/b821698c
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The creation of a sustainable energy generation, storage, and distribution infrastructure represents a global grand challenge that requires massive transnational investments in the research and development of energy technologies that will provide the amount of energy needed on a sufficient scale and timeframe with minimal impact on the environment and have limited economic and societal disruption during implementation. In this opinion paper, we focus on an important set of solar, thermal, and electrochemical energy conversion, storage, and conservation technologies specifically related to recent and prospective advances in nanoscale science and technology that offer high potential in addressing the energy challenge. We approach this task from a two-fold perspective: analyzing the fundamental physicochemical principles and engineering aspects of these energy technologies and identifying unique opportunities enabled by nanoscale design of materials, processes, and systems in order to improve performance and reduce costs. Our principal goal is to establish a roadmap for research and development activities in nanoscale science and technology that would significantly advance and accelerate the implementation of renewable energy technologies. In all cases we make specific recommendations for research needs in the near-term (2-5 years), mid-term (5-10 years) and long-term (>10 years), as well as projecting a timeline for maturation of each technological solution. We also identify a number of priority themes in basic energy science that cut across the entire spectrum of energy conversion, storage, and conservation technologies. We anticipate that the conclusions and recommendations herein will be of use not only to the technical community, but also to policy makers and the broader public, occasionally with an admitted emphasis on the US perspective.
引用
收藏
页码:559 / 588
页数:30
相关论文
共 224 条
[1]   Vehicular storage of hydrogen in insulated pressure vessels [J].
Aceves, Salvador M. ;
Berry, Gene D. ;
Martinez-Frias, Joel ;
Espinosa-Loza, Francisco .
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2006, 31 (15) :2274-2283
[2]   Silicon oxide Nafion composite membranes for proton-exchange membrane fuel cell operation at 80-140° C [J].
Adjemian, KT ;
Lee, SJ ;
Srinivasan, S ;
Benziger, J ;
Bocarsly, AB .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2002, 149 (03) :A256-A261
[3]   Synthesis of colloidal magnesium:: A near room temperature store for hydrogen [J].
Aguey-Zinsou, Kondo-Francois ;
Ares-Fernandez, Jose-Ramon .
CHEMISTRY OF MATERIALS, 2008, 20 (02) :376-378
[4]   Using first principles calculations to identify new destabilized metal hydride reactions for reversible hydrogen storage [J].
Alapati, Sudhakar V. ;
Johnson, J. Karl ;
Sholl, David S. .
PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2007, 9 (12) :1438-1452
[5]   Fluoride based electrode materials for advanced energy storage devices [J].
Amatucci, Glenn G. ;
Pereira, Nathalie .
JOURNAL OF FLUORINE CHEMISTRY, 2007, 128 (04) :243-262
[6]   ESD FAILURE MODES - CHARACTERISTICS, MECHANISMS, AND PROCESS INFLUENCES [J].
AMERASEKERA, A ;
VANDENABEELEN, W ;
VANROOZENDAAL, L ;
HANNEMANN, M ;
SCHOFIELD, P .
IEEE TRANSACTIONS ON ELECTRON DEVICES, 1992, 39 (02) :430-436
[7]   Measurement of SO2 solubility in ionic liquids [J].
Anderson, Jessica L. ;
Dixon, JaNeille K. ;
Maginn, Edward J. ;
Brennecke, Joan F. .
JOURNAL OF PHYSICAL CHEMISTRY B, 2006, 110 (31) :15059-15062
[8]  
Anderson ML, 2002, NANO LETT, V2, P235, DOI 10.1021/n1015707d
[9]  
[Anonymous], 2005, Avoiding Dangerous Climate Change
[10]  
[Anonymous], 2003, HDB FUEL CELLS FUNDA