Tunneling of a large spin via hyperfine interactions

被引:28
作者
Garanin, DA
Chudnovsky, EM
Schilling, R
机构
[1] Max Planck Inst Phys Complexer Syst, D-01187 Dresden, Germany
[2] CUNY Herbert H Lehman Coll, Dept Phys & Astron, Bronx, NY 10468 USA
[3] Univ Mainz, Inst Phys, D-6500 Mainz, Germany
来源
PHYSICAL REVIEW B | 2000年 / 61卷 / 18期
基金
美国国家科学基金会;
关键词
D O I
10.1103/PhysRevB.61.12204
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We consider a large spin S in the magnetic field parallel to the uniaxial crystal field, interacting with N much greater than 1 nuclear spins Ii via Hamiltonian H=-DSz2+HzSz+AS .Sigma(i=1)(N)I(i) with A much less than D, at temperature T. Tunneling splittings and the selection rules for the resonant values of H-z are obtained perturbatively. The quantum coherence exists at T much less than ASI while at T greater than or similar to ASI the coherence is destroyed and the relaxation of S is described by a stretched dependence which can be close to log t under certain conditions. Relevance to Mn-12 acetate is discussed.
引用
收藏
页码:12204 / 12208
页数:5
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