State-to-state exciton dynamics in semiconductor quantum dots

被引:158
作者
Sewall, Samuel L. [1 ]
Cooney, Ryan R. [1 ]
Anderson, Kevin E. H. [1 ]
Dias, Eva A. [1 ]
Kambhampati, Patanjali [1 ]
机构
[1] McGill Univ, Dept Chem, Montreal, PQ H3A 2K6, Canada
关键词
D O I
10.1103/PhysRevB.74.235328
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Femtosecond carrier relaxation dynamics in colloidal CdSe quantum dots are measured which focus on the early time dynamics for different initial excitonic states. Selecting the initial excitonic states produces a clear influence upon the early time dynamics. The difference between the dynamics when initially populating different excitonic states provides a direct measurement of excitonic relaxation times in strongly confined colloidal semiconductor quantum dots with specificity to electrons and holes. These results furthermore show state specific biexciton interactions.
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页数:8
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共 27 条
[21]   Exciton molecules in multi-valley semiconductors [J].
Rogachev, AA .
PROGRESS IN QUANTUM ELECTRONICS, 2001, 25 (04) :141-164
[22]   STARK SPECTROSCOPY OF CDSE NANOCRYSTALLITES - THE SIGNIFICANCE OF TRANSITION LINEWIDTHS [J].
SACRA, A ;
NORRIS, DJ ;
MURRAY, CB ;
BAWENDI, MG .
JOURNAL OF CHEMICAL PHYSICS, 1995, 103 (13) :5236-5245
[23]  
SEWALL SL, UNPUB
[24]   Femtosecond multicolor pump-probe study of ultrafast electron transfer of [(NH3)5RuIIINCRuII(CN)5]- in aqueous solution [J].
Son, DH ;
Kambhampati, P ;
Kee, TW ;
Barbara, PF .
JOURNAL OF PHYSICAL CHEMISTRY A, 2002, 106 (18) :4591-4597
[25]   Pseudopotential theory of Auger processes in CdSe quantum dots [J].
Wang, LW ;
Califano, M ;
Zunger, A ;
Franceschetti, A .
PHYSICAL REVIEW LETTERS, 2003, 91 (05)
[26]   Huge binding energy of localized biexcitons in CdS/ZnS quantum structures [J].
Woggon, U ;
Hild, K ;
Gindele, F ;
Langbein, W ;
Hetterich, M ;
Grün, M ;
Klingshirn, C .
PHYSICAL REVIEW B, 2000, 61 (19) :12632-12635
[27]   Experimental determination of the extinction coefficient of CdTe, CdSe, and CdS nanocrystals [J].
Yu, WW ;
Qu, LH ;
Guo, WZ ;
Peng, XG .
CHEMISTRY OF MATERIALS, 2003, 15 (14) :2854-2860