Anisotropic exchange in frustrated pyrochlore Yb2Ti2O7

被引:39
作者
Cao, H. B. [2 ]
Gukasov, A. [2 ]
Mirebeau, I. [2 ]
Bonville, P. [1 ]
机构
[1] CEA, Ctr Saclay, IRAMIS, Serv Phys Etat Condense, F-91191 Gif Sur Yvette, France
[2] CEA, Ctr Saclay, Lab Leon Brillouin, F-91191 Gif Sur Yvette, France
关键词
CRYSTAL-FIELD;
D O I
10.1088/0953-8984/21/49/492202
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
The local Yb3+ magnetic susceptibility tensor was recently measured in the frustrated pyrochlore compound Yb2Ti2O7 by means of in-field polarized neutron scattering in a single crystal. A very anisotropic effective exchange tensor was derived for the Yb3+ ion. Using this result, we reinterpret here the data for the powder susceptibility in Yb2Ti2O7. We show that, in the case of a well-isolated Kramers doublet with anisotropic g and exchange tensors, the inverse susceptibility for a powder sample does not strictly obey a Curie-Weiss law at low temperature. We discuss the consequences regarding the paramagnetic Curie temperature, usually taken as a measure of the exchange/dipolar interaction, and the exotic 'slow fluctuation' ground state of Yb2Ti2O7.
引用
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页数:5
相关论文
共 28 条
[1]  
ABRAGAM A, 1969, ELECT PARAMAGNETIC R
[2]   QUADRUPOLE INTERACTIONS AND RELAXATION EFFECTS IN DY2TI2O7 [J].
ALMOG, A ;
BAUMINGER, ER ;
LEVY, A ;
NOWIK, I ;
OFER, S .
SOLID STATE COMMUNICATIONS, 1973, 12 (07) :693-696
[3]  
BERT F, 2006, PHYS REV LETT, V96
[4]   HEAT-CAPACITY MEASUREMENTS ON RARE-EARTH DOUBLE OXIDES R2M2O7 [J].
BLOTE, HWJ ;
WIELINGA, RF ;
HUISKAMP, WJ .
PHYSICA, 1969, 43 (04) :549-&
[5]   Transitions and spin dynamics at very low temperature in the pyrochlores Yb2Ti2O7 and Gd2Sn2O7 [J].
Bonville, P ;
Hodges, JA ;
Bertin, E ;
Bouchaud, JP ;
De Réotier, PD ;
Regnault, LP ;
Ronnow, HM ;
Sanchez, JP ;
Sosin, S ;
Yaouanc, A .
HYPERFINE INTERACTIONS, 2004, 156 (01) :103-111
[6]  
BONVILLE P, 2003, P 38 ZAK C KRAK
[7]   Ising versus XY Anisotropy in Frustrated R2Ti2O7 Compounds as "Seen'' by Polarized Neutrons [J].
Cao, H. ;
Gukasov, A. ;
Mirebeau, I. ;
Bonville, P. ;
Decorse, C. ;
Dhalenne, G. .
PHYSICAL REVIEW LETTERS, 2009, 103 (05)
[8]   Spin dynamics and magnetic order in magnetically frustrated Tb2Sn2O7 [J].
de Réotier, PD ;
Yaouanc, A ;
Keller, L ;
Cervellino, A ;
Roessli, B ;
Baines, C ;
Forget, A ;
Vaju, C ;
Gubbens, PCM ;
Amato, A ;
King, PJC .
PHYSICAL REVIEW LETTERS, 2006, 96 (12)
[9]   Dynamical crossover in 'hot' spin ice [J].
Ehlers, G ;
Cornelius, AL ;
Orendác, M ;
Kajnaková, M ;
Fennell, T ;
Bramwell, ST ;
Gardner, JS .
JOURNAL OF PHYSICS-CONDENSED MATTER, 2003, 15 (02) :L9-L15
[10]   Spin-spin correlations in Yb2Ti2O7:: A polarized neutron scattering study -: art. no. 180404 [J].
Gardner, JS ;
Ehlers, G ;
Rosov, N ;
Erwin, RW ;
Petrovic, C .
PHYSICAL REVIEW B, 2004, 70 (18) :1-4