Anisotropic exchange in frustrated pyrochlore Yb2Ti2O7

被引:39
作者
Cao, H. B. [2 ]
Gukasov, A. [2 ]
Mirebeau, I. [2 ]
Bonville, P. [1 ]
机构
[1] CEA, Ctr Saclay, IRAMIS, Serv Phys Etat Condense, F-91191 Gif Sur Yvette, France
[2] CEA, Ctr Saclay, Lab Leon Brillouin, F-91191 Gif Sur Yvette, France
关键词
CRYSTAL-FIELD;
D O I
10.1088/0953-8984/21/49/492202
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
The local Yb3+ magnetic susceptibility tensor was recently measured in the frustrated pyrochlore compound Yb2Ti2O7 by means of in-field polarized neutron scattering in a single crystal. A very anisotropic effective exchange tensor was derived for the Yb3+ ion. Using this result, we reinterpret here the data for the powder susceptibility in Yb2Ti2O7. We show that, in the case of a well-isolated Kramers doublet with anisotropic g and exchange tensors, the inverse susceptibility for a powder sample does not strictly obey a Curie-Weiss law at low temperature. We discuss the consequences regarding the paramagnetic Curie temperature, usually taken as a measure of the exchange/dipolar interaction, and the exotic 'slow fluctuation' ground state of Yb2Ti2O7.
引用
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页数:5
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