Recombination dynamics of excitons in Mg0.11Zn0.89O alloy films grown using the high-temperature-annealed self-buffer layer by laser-assisted molecular-beam epitaxy

被引:24
作者
Kubota, Masashi
Onuma, Takeyoshi
Tsukazaki, Atsushi
Ohtomo, Akira
Kawasaki, Masashi
Sota, Takayuki
Chichibu, Shigefusa F. [1 ]
机构
[1] Tohoku Univ, Inst Multidisciplinary Res Adv Mat, Sendai, Miyagi 9808577, Japan
[2] Univ Tsukuba, Inst Appl Phys, Tsukuba, Ibaraki 3058573, Japan
[3] Univ Tsukuba, Century COE Off 21st, Tsukuba, Ibaraki 3058573, Japan
[4] JST, ERATO, Nakamura Inhomogeneous Crystal Project, Kawaguchi 3320012, Japan
关键词
ZNO; PHOTOLUMINESCENCE;
D O I
10.1063/1.2719168
中图分类号
O59 [应用物理学];
学科分类号
摘要
Recombination dynamics of excitons in Mg0.11Zn0.89O epilayers grown by laser-assisted molecular-beam epitaxy on a ScAlMgO4 substrate were investigated. By using the MgZnO high-temperature-annealed self-buffer layer (HITAB), the value of full width at half maximum of the near-band-edge (NBE) photoluminescence (PL) peak at 3.6 eV was decreased from 133 to 94 meV at 293 K, and the intensity ratio of the NBE emission to the deep emission band centered around 2.2 eV was increased by a factor of 3. Also, the PL lifetime of the NBE peak at 293 K under the excitation density of 1 mu J/cm(2) was increased from 49 to 60 ps. These results suggest that HITAB gave rise to improved alloy compositional homogeneity and reduced concentration of point defects.
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页数:3
相关论文
共 18 条
[1]   THERMALIZATION EFFECT ON RADIATIVE DECAY OF EXCITONS IN QUANTUM WIRES [J].
AKIYAMA, H ;
KOSHIBA, S ;
SOMEYA, T ;
WADA, K ;
NOGE, H ;
NAKAMURA, Y ;
INOSHITA, T ;
SHIMIZU, A ;
SAKAKI, H .
PHYSICAL REVIEW LETTERS, 1994, 72 (06) :924-927
[2]   Improvements in quantum efficiency of excitonic emissions in ZnO epilayers by the elimination of point defects [J].
Chichibu, S. F. ;
Onuma, T. ;
Kubota, M. ;
Uedono, A. ;
Sota, T. ;
Tsukazaki, A. ;
Ohtomo, A. ;
Kawasaki, M. .
JOURNAL OF APPLIED PHYSICS, 2006, 99 (09)
[3]   Exciton-polariton spectra and limiting factors for the room-temperature photoluminescence efficiency in ZnO [J].
Chichibu, SF ;
Uedono, A ;
Tsukazaki, A ;
Onuma, T ;
Zamfirescu, M ;
Ohtomo, A ;
Kavokin, A ;
Cantwell, G ;
Litton, CW ;
Sota, T ;
Kawasaki, M .
SEMICONDUCTOR SCIENCE AND TECHNOLOGY, 2005, 20 (04) :S67-S77
[4]   RAMAN EFFECT IN ZINC OXIDE [J].
DAMEN, TC ;
PORTO, SPS ;
TELL, B .
PHYSICAL REVIEW, 1966, 142 (02) :570-&
[5]   LINEWIDTH DEPENDENCE OF RADIATIVE EXCITON LIFETIMES IN QUANTUM-WELLS [J].
FELDMANN, J ;
PETER, G ;
GOBEL, EO ;
DAWSON, P ;
MOORE, K ;
FOXON, C ;
ELLIOTT, RJ .
PHYSICAL REVIEW LETTERS, 1987, 59 (20) :2337-2340
[6]   p-type electrical conduction in ZnO thin films by Ga and N codoping [J].
Joseph, M ;
Tabata, H ;
Kawai, T .
JAPANESE JOURNAL OF APPLIED PHYSICS PART 2-LETTERS & EXPRESS LETTERS, 1999, 38 (11A) :L1205-L1207
[7]   In situ monitoring of Zn* and Mg* species during helicon-wave-excited-plasma sputtering epitaxy of ZnO and Mg0.06Zn0.94O films [J].
Koyama, T ;
Ohmori, T ;
Shibata, N ;
Onuma, T ;
Chichibu, SF .
JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B, 2004, 22 (04) :2220-2225
[8]   Characterization of homoepitaxial p-type ZnO grown by molecular beam epitaxy [J].
Look, DC ;
Reynolds, DC ;
Litton, CW ;
Jones, RL ;
Eason, DB ;
Cantwell, G .
APPLIED PHYSICS LETTERS, 2002, 81 (10) :1830-1832
[9]   Growth of p-type zinc oxide films by chemical vapor deposition [J].
Minegishi, K ;
Koiwai, Y ;
Kikuchi, Y ;
Yano, K ;
Kasuga, M ;
Shimizu, A .
JAPANESE JOURNAL OF APPLIED PHYSICS PART 2-LETTERS & EXPRESS LETTERS, 1997, 36 (11A) :L1453-L1455
[10]   Photoluminescence from exciton-exciton scattering in a lightly alloyed InGaN thin film under intense excitation conditions [J].
Nakayama, M ;
Kitano, R ;
Ando, M ;
Uemura, T .
APPLIED PHYSICS LETTERS, 2005, 87 (09)