Impact of the mixing boundary layer on the relationship between PM2.5 and aerosol optical thickness

被引:58
作者
Boyouk, Neda [1 ,2 ,3 ]
Leon, Jean-Francois [1 ,2 ,3 ]
Delbarre, Herve [1 ,4 ,5 ]
Podvin, T. [1 ,2 ,3 ]
Deroo, C. [1 ,2 ,3 ]
机构
[1] Univ Lille Nord France, F-59000 Lille, France
[2] USTL, LOA, F-59655 Villeneuve Dascq, France
[3] CNRS, UMR 8518, F-59655 Villeneuve Dascq, France
[4] ULCO, LPCA, F-59140 Dunkerque, France
[5] CNRS, UMR 8101, F-59140 Dunkerque, France
关键词
Mass concentration; Aerosol optical thickness; Boundary layer; Lidar; COMPLEX REFRACTIVE-INDEX; PARTICULATE MATTER; AIR-POLLUTION; LIDAR; URBAN; RETRIEVAL; NETWORK; AERONET; HEIGHT; SUN;
D O I
10.1016/j.atmosenv.2009.06.053
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The purpose of this paper is to study the relationship between columnar aerosol optical thickness and ground-level aerosol mass. A set of Sun photometer, elastic backscattering lidar and TEOM measurements were acquired during April 2007 in Lille, France. The PM2.5 in the mixed boundary layer is estimated using the lidar signal, aerosol optical thickness, or columnar integrated Sun photometer size distribution and compared to the ground-level station measurements. The lidar signal recorded in the lowest level (240 m) is well correlated to the PM2.5 (R-2 = 0.84). We also show that the correlation between AOT-derived and measured PM2.5 is significantly improved when considering the mixed boundary layer height derived from the lidar. The use of the Sun photometer aerosol fine fraction volume does not improve the correlation. (C) 2009 Elsevier Ltd. All rights reserved.
引用
收藏
页码:271 / 277
页数:7
相关论文
共 40 条
[1]   Evaluation of the TEOM(R) method for measurement of ambient particulate mass in urban areas [J].
Allen, G ;
Sioutas, C ;
Koutrakis, P ;
Reiss, R ;
Lurmann, FW ;
Roberts, PT .
JOURNAL OF THE AIR & WASTE MANAGEMENT ASSOCIATION, 1997, 47 (06) :682-689
[2]   European pollution outbreaks during ACE 2:: Lofted aerosol plumes observed with Raman lidar at the Portuguese coast [J].
Ansmann, A ;
Wagner, F ;
Althausen, D ;
Müller, D ;
Herber, A ;
Wandinger, U .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2001, 106 (D18) :20725-20733
[3]  
Ansmann A., 2005, Lidar. Range-Resolved Optical Remote Sensing of the Atmosphere, P105, DOI [10.1007/0-387-25101-4_4, DOI 10.1007/0-387-25101-4_4]
[4]   Continuous monitoring of the boundary-layer top with lidar [J].
Baars, H. ;
Ansmann, A. ;
Engelmann, R. ;
Althausen, D. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2008, 8 (23) :7281-7296
[5]   Variability of aerosol and spectral lidar and backscatter and extinction ratios of key aerosol types derived from selected Aerosol Robotic Network locations [J].
Cattrall, C ;
Reagan, J ;
Thome, K ;
Dubovik, O .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2005, 110 (D10) :1-13
[6]   Global monitoring of air pollution over land from the Earth Observing System-Terra Moderate Resolution Imaging Spectroradiometer (MODIS) [J].
Chu, DA ;
Kaufman, YJ ;
Zibordi, G ;
Chern, JD ;
Mao, J ;
Li, CC ;
Holben, BN .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2003, 108 (D21)
[7]  
Dockery D.W., 1993, N ENGL J MED, V329
[8]   Accuracy assessments of aerosol optical properties retrieved from Aerosol Robotic Network (AERONET) Sun and sky radiance measurements [J].
Dubovik, O ;
Smirnov, A ;
Holben, BN ;
King, MD ;
Kaufman, YJ ;
Eck, TF ;
Slutsker, I .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2000, 105 (D8) :9791-9806
[9]   A flexible inversion algorithm for retrieval of aerosol optical properties from Sun and sky radiance measurements [J].
Dubovik, O ;
King, MD .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2000, 105 (D16) :20673-20696
[10]  
Dubovik O, 2002, J ATMOS SCI, V59, P590, DOI 10.1175/1520-0469(2002)059<0590:VOAAOP>2.0.CO