Four-photon absorption in the single-crystal polymer bis(paratoluene) sulfonate

被引：29

作者：

Shim, H ^{[1
]}

Liu, MG ^{[1
]}

Hwangbo, CK ^{[1
]}

Stegeman, GI ^{[1
]}

机构：

[1] Univ Cent Florida, Ctr Res & Educ Opt & Lasers, Orlando, FL 32816 USA

来源：

OPTICS LETTERS | 1998年 / 23卷 / 06期

关键词：

D O I：

10.1364/OL.23.000430

中图分类号：

O43 [光学];

学科分类号：

070207 ; 0803 ;

摘要：

Strong four-photon absorption corresponding to Im[chi((tau))((-)omega; w, (-)omega, omega, (-)omega, omega, (-)omega, omega)] has been measured for the first time to the authors' knowledge with 100-fs pulses at 1600 nm in the single-crystal polymer poly[bis(p-toluene sulfonate)] of 2,4-hexadiyne-1,6-diol. The transition involved is from the even-symmetry ground state into the vibronic subband of the dominant, even-symmetry, excited two-photon state at an energy of 2.7 eV. (C) 1998 Optical Society of America.

引用

页码：430 / 432

页数：3

共 16 条

[1] THE PICOSECOND SPECTROSCOPY OF A POLYDIACETYLENE IN THE SMALL-SIGNAL LIMIT - DETECTION AND CHARACTERIZATION OF A NEW LONG-LIVED STATE [J].

BLANCHARD, GJ ;

HERITAGE, JP ;

BAKER, GL ;

ETEMAD, S .

CHEMICAL PHYSICS LETTERS, 1989, 158 (3-4) :329-333

[2]

BLOEMBERGEN N, 1997, COMMUNICATION

[3]

ETEMAD S, 1994, MOL NONLINEAR OPTICS, P433

[4] Scaling of four-photon absorption in InAs [J].

Hasselbeck, MP ;

VanStryland, EW ;

SheikBahae, M .

JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS, 1997, 14 (07) :1616-1624

[5]

HE S, 1995, OPT LETT, V20, P1524

[6] ASSESSMENT OF SINGLE-CRYSTAL P-TOLUENE SULFONATE AS AN ALL-OPTICAL SWITCHING MATERIAL AT 1.3-MU-M [J].

KIM, DY ;

LAWRENCE, BL ;

TORRUELLAS, WE ;

STEGEMAN, GI ;

BAKER, G ;

METH, J .

APPLIED PHYSICS LETTERS, 1994, 65 (14) :1742-1744

[7] IDENTIFICATION AND ROLE OF 2-PHOTON-EXCITED STATES IN A PI-CONJUGATED POLYMER [J].

LAWRENCE, B ;

TORRUELLAS, WE ;

CHA, M ;

SUNDHEIMER, ML ;

STEGEMAN, GI ;

METH, J ;

ETEMAD, S ;

BAKER, G .

PHYSICAL REVIEW LETTERS, 1994, 73 (04) :597-600

[8] MEASUREMENT OF THE COMPLEX NONLINEAR REFRACTIVE-INDEX OF SINGLE-CRYSTAL P-TOLUENE SULFONATE AT 1064-NM [J].

LAWRENCE, BL ;

CHA, M ;

TORRUELLAS, WE ;

STEGEMAN, GI ;

ETEMAD, S ;

BAKER, G ;

KAJZAR, F .

APPLIED PHYSICS LETTERS, 1994, 64 (21) :2773-2775

[9] LARGE PURELY REFRACTIVE NONLINEAR INDEX OF SINGLE-CRYSTAL P-TOLUENE SULFONATE (PTS) AT 1600 NM [J].

LAWRENCE, BL ;

CHA, M ;

KANG, JU ;

TORUELLAS, W ;

STEGEMAN, G ;

BAKER, G ;

METH, J ;

ETEMAD, S .

ELECTRONICS LETTERS, 1994, 30 (05) :447-448

[10] OPTICAL NONLINEARITIES IN ONE-DIMENSIONAL-CONJUGATED POLYMER CRYSTALS [J].

SAUTERET, C ;

HERMANN, JP ;

FREY, R ;

PRADERE, F ;

DUCUING, J ;

BAUGHMAN, RH ;

CHANCE, RR .

PHYSICAL REVIEW LETTERS, 1976, 36 (16) :956-959

← 1 2 →