The effect of temperature on the removal of DCM using non-thermal, atmospheric-pressure plasma-assisted catalysis

被引:15
作者
Harling, Alice M. [1 ]
Wallis, Anna E. [1 ]
Whitehead, J. Christopher [1 ]
机构
[1] Univ Manchester, Sch Chem, Manchester M13 9PL, Lancs, England
关键词
AC barrier discharges; catalysis; dichloromethane; environmental clean-up; FT-IR; non-thermal plasma;
D O I
10.1002/ppap.200600207
中图分类号
O59 [应用物理学];
学科分类号
摘要
A non-thermal, atmospheric-pressure plasma has been used to study the effect of temperature on the plasma destruction of DCM in an air stream using a BaTiO3-packed-bedreactor, co-filled with TiO2 and gamma-Al2O3 catalysts. Comparisons have been made with plasma alone, catalysis alone and combined plasma/catalysis to determine any synergistic effects of combininig plasma and catalysis. Plasma/catalysis is the most successful method for destroying DCM over 125-400 degrees C. TiO2 was more effective than gamma-Al2O3 for plasma/catalysis. The energy efficiency of plasma/catalysis processing compared to catalysis alone is considered by examining the input power required to achieve equivalent destructions, finding that an energy reduction of approximate to 30% can be achieved by plasma activation of the catalyst.
引用
收藏
页码:463 / 470
页数:8
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