KINETICS OF OXYGEN-INDUCED FACETING OF VICINAL AG(110)

被引:79
作者
OZCOMERT, JS [1 ]
PAI, WW [1 ]
BARTELT, NC [1 ]
REUTTROBEY, JE [1 ]
机构
[1] UNIV MARYLAND,DEPT CHEM,COLL PK,MD 20742
关键词
D O I
10.1103/PhysRevLett.72.258
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The oxygen-induced breakup of vicinal Ag(110) surfaces into (110) facets and step bunches is measured with scanning tunneling microscopy. Faceting transitions are recorded in real time at room temperature for two surface orientations. A vicinal Ag(110) surface misoriented by 2-degrees towards [001] facets via the growth of isolated nuclei. Step-position fluctuations of increasing magnitude are observed prior to faceting, revealing a critical terrace width of approximately 100 angstrom. In contrast, oxygen exposure causes Ag(110) misoriented by 2-degrees towards [331BAR] to facet spontaneously with no evident nucleation barrier.
引用
收藏
页码:258 / 261
页数:4
相关论文
共 23 条
[1]  
Chernov A., 1961, SOV PHYS USP, V4, P116, DOI [DOI 10.1070/PU1961V004N01ABEH003328, 10.1070/PU1961v004n01ABEH003328.]
[2]   ADSORPTION OF OXYGEN ON SILVER SINGLE-CRYSTAL SURFACES [J].
ENGELHARDT, HA ;
MENZEL, D .
SURFACE SCIENCE, 1976, 57 (02) :591-618
[3]   MORPHOLOGY AND ETCHING PROCESSES ON MACROSCOPIC METAL-CATALYSTS [J].
FLYTZANI-STEPHANOPOULOS, M ;
SCHMIDT, LD .
PROGRESS IN SURFACE SCIENCE, 1979, 9 (03) :83-111
[4]   FRIZZED APPEARANCE OF STEPS IN TUNNEL MICROSCOPY ON CU(100) AND VICINAL CU(11N) SURFACES [J].
GIESEN, M ;
FROHN, J ;
POENSGEN, M ;
WOLF, JF ;
IBACH, H .
JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A-VACUUM SURFACES AND FILMS, 1992, 10 (04) :2597-2599
[5]   SOME THEOREMS ON THE FREE ENERGIES OF CRYSTAL SURFACES [J].
HERRING, C .
PHYSICAL REVIEW, 1951, 82 (01) :87-93
[6]   HIGH-TEMPERATURE SCANNING-TUNNELING-MICROSCOPY OBSERVATION OF PHASE-TRANSITIONS AND RECONSTRUCTION ON A VICINAL SI(111) SURFACE [J].
HIBINO, H ;
FUKUDA, T ;
SUZUKI, M ;
HOMMA, Y ;
SATO, T ;
IWATSUKI, M ;
MIKI, K ;
TOKUMOTO, H .
PHYSICAL REVIEW B, 1993, 47 (19) :13027-13030
[7]   THE STABILITY OF ULTRATHIN METAL-FILMS ON W(110) AND W(111) [J].
MADEY, TE ;
SONG, KJ ;
DONG, CZ ;
DEMMIN, RA .
SURFACE SCIENCE, 1991, 247 (2-3) :175-187
[8]   ADSORPTION-DESORPTION PROPERTIES, COADSORPTION, AND SURFACE STRUCTURAL CHEMISTRY OF CHLORINE AND OXYGEN ON AG(331) [J].
MARBROW, RA ;
LAMBERT, RM .
SURFACE SCIENCE, 1978, 71 (01) :107-120
[9]  
MOORE AJW, 1962, METAL SURFACES, P155
[10]   THEORY OF LINEAR FACET GROWTH DURING THERMAL ETCHING [J].
MULLINS, WW .
PHILOSOPHICAL MAGAZINE, 1961, 6 (71) :1313-1341