Mapping the spatial distribution of charge carriers in LaAlO3/SrTiO3 heterostructures

被引:363
作者
Basletic, M. [1 ]
Maurice, J. -L. [1 ]
Carretero, C. [1 ]
Herranz, G. [1 ]
Copie, O. [1 ]
Bibes, M. [1 ]
Jacquet, E. [1 ]
Bouzehouane, K. [1 ]
Fusil, S. [1 ]
Barthelemy, A. [1 ]
机构
[1] Univ Paris Sud, CNRS Thales, Unite Mixte Phys, F-91767 Palaiseau, France
关键词
D O I
10.1038/nmat2223
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
At the interface between complex insulating oxides, novel phases with interesting properties may occur, such as the metallic state reported in the LaAlO(3)/SrTiO(3) system(1). Although this state has been predicted(2) and reported(3,4) to be confined at the interface, some studies indicate a much broader spatial extension(5), thereby questioning its origin. Here, we provide for the first time a direct determination of the carrier density profile of this system through resistance profile mappings collected in cross-section LaAlO(3)/SrTiO(3) samples with a conducting-tip atomic force microscope (CT-AFM). We find that, depending on specific growth protocols, the spatial extension of the high-mobility electron gas can be varied from hundreds of micrometres into SrTiO(3) to a few nanometres next to the LaAlO(3)/SrTiO(3) interface. Our results emphasize the potential of CT-AFM as a novel tool to characterize complex oxide interfaces and provide us with a definitive and conclusive way to reconcile the body of experimental data in this system.
引用
收藏
页码:621 / 625
页数:5
相关论文
共 26 条
[1]   Enhanced dielectric properties of SrTiO3 epitaxial thin film for tunable microwave devices [J].
Bouzehouane, K ;
Woodall, P ;
Marcilhac, B ;
Khodan, AN ;
Crété, D ;
Jacquet, E ;
Mage, JC ;
Contour, JP .
APPLIED PHYSICS LETTERS, 2002, 80 (01) :109-111
[2]   Magnetic effects at the interface between non-magnetic oxides [J].
Brinkman, A. ;
Huijben, M. ;
Van Zalk, M. ;
Huijben, J. ;
Zeitler, U. ;
Maan, J. C. ;
Van der Wiel, W. G. ;
Rijnders, G. ;
Blank, D. H. A. ;
Hilgenkamp, H. .
NATURE MATERIALS, 2007, 6 (07) :493-496
[3]   Nanoscale control of an interfacial metal-insulator transition at room temperature [J].
Cen, C. ;
Thiel, S. ;
Hammerl, G. ;
Schneider, C. W. ;
Andersen, K. E. ;
Hellberg, C. S. ;
Mannhart, J. ;
Levy, J. .
NATURE MATERIALS, 2008, 7 (04) :298-302
[4]   Oxide interfaces - Watch out for the lack of oxygen [J].
Eckstein, James N. .
NATURE MATERIALS, 2007, 6 (07) :473-474
[5]   Photoemission (XPS and XPD) study of epitaxial LaAlO3 fiim grown on SrTiO3(001) [J].
El Kazzi, M. ;
Merckling, C. ;
Delhaye, G. ;
Arzel, L. ;
Grenet, G. ;
Bergignat, E. ;
Hollinger, G. .
MATERIALS SCIENCE IN SEMICONDUCTOR PROCESSING, 2006, 9 (06) :954-958
[6]   HALL MOBILITY IN SRTIO3 [J].
FREDERIKSE, HP ;
HOSLER, WR .
PHYSICAL REVIEW, 1967, 161 (03) :822-+
[7]   High mobility in LaAlO3/SrTiO3 heterostructures:: Origin, dimensionality, and perspectives [J].
Herranz, G. ;
Basletic, M. ;
Bibes, M. ;
Carretero, C. ;
Tafra, E. ;
Jacquet, E. ;
Bouzehouane, K. ;
Deranlot, C. ;
Hamzic, A. ;
Broto, J.-M. ;
Barthelemy, A. ;
Fert, A. .
PHYSICAL REVIEW LETTERS, 2007, 98 (21)
[8]   Imaging the local electrical properties of metal surfaces by atomic force microscopy with conducting probes [J].
Houze, F ;
Meyer, R ;
Schneegans, O ;
Boyer, L .
APPLIED PHYSICS LETTERS, 1996, 69 (13) :1975-1977
[9]   Electronically coupled complementary interfaces between perovskite band insulators [J].
Huijben, Mark ;
Rijnders, Guus ;
Blank, Dave H. A. ;
Bals, Sara ;
Van Aert, Sandra ;
Verbeeck, Jo ;
Van Tendeloo, Gustaaf ;
Brinkman, Alexander ;
Hilgenkamp, Hans .
NATURE MATERIALS, 2006, 5 (07) :556-560
[10]   DIFFUSION OF OXIDE ION VACANCIES IN PEROVSKITE-TYPE OXIDES [J].
ISHIGAKI, T ;
YAMAUCHI, S ;
KISHIO, K ;
MIZUSAKI, J ;
FUEKI, K .
JOURNAL OF SOLID STATE CHEMISTRY, 1988, 73 (01) :179-187