Interplay between thermodynamics and kinetics in the capping of InAs/GaAs(001) quantum dots

被引:122
作者
Costantini, G. [1 ]
Rastelli, A. [1 ]
Manzano, C. [1 ]
Acosta-Diaz, P. [1 ]
Songmuang, R. [1 ]
Katsaros, G. [1 ]
Schmidt, O. G. [1 ]
Kern, K. [1 ]
机构
[1] Max Planck Inst Festkorperforsch, D-70569 Stuttgart, Germany
关键词
D O I
10.1103/PhysRevLett.96.226106
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
A microscopic picture for the GaAs overgrowth of self-organized InAs/GaAs(001) quantum dots is developed. Scanning tunneling microscopy measurements reveal two capping regimes: the first being characterized by a dot shrinking and a backward pyramid-to-dome shape transition. This regime is governed by fast dynamics resulting in island morphologies close to thermodynamic equilibrium. The second regime is marked by a true overgrowth and is controlled by kinetically limited surface diffusion processes. A simple model is developed to describe the observed structural changes which are rationalized in terms of energetic minimization driven by lattice mismatch and alloying.
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页数:4
相关论文
共 29 条
[1]   Surface alloying at InAs-GaAs interfaces grown on (001) surfaces by molecular beam epitaxy [J].
Belk, JG ;
McConville, CF ;
Sudijono, JL ;
Jones, TS ;
Joyce, BA .
SURFACE SCIENCE, 1997, 387 (1-3) :213-226
[2]  
Bimberg D., 1999, QUANTUM DOT HETEROST
[3]   Wetting droplet instability and quantum ring formation [J].
Blossey, R ;
Lorke, A .
PHYSICAL REVIEW E, 2002, 65 (02)
[4]   Determination of the shape and indium distribution of low-growth-rate InAs quantum dots by cross-sectional scanning tunneling microscopy [J].
Bruls, DM ;
Vugs, JWAM ;
Koenraad, PM ;
Salemink, HWM ;
Wolter, JH ;
Hopkinson, M ;
Skolnick, MS ;
Long, F ;
Gill, SPA .
APPLIED PHYSICS LETTERS, 2002, 81 (09) :1708-1710
[5]   Pyramids and domes in the InAs/GaAs(001) and Ge/Si(001) systems [J].
Costantini, G ;
Rastelli, A ;
Manzano, C ;
Acosta-Diaz, P ;
Katsaros, G ;
Songmuang, R ;
Schmidt, OG ;
Von Känel, H ;
Kern, K .
JOURNAL OF CRYSTAL GROWTH, 2005, 278 (1-4) :38-45
[6]   Universal shapes of self-organized semiconductor quantum dots:: Striking similarities between InAs/GaAs(001) and Ge/Si(001) [J].
Costantini, G ;
Rastelli, A ;
Manzano, C ;
Songmuang, R ;
Schmidt, OG ;
Kern, K ;
von Känel, H .
APPLIED PHYSICS LETTERS, 2004, 85 (23) :5673-5675
[7]   Lateral motion of SiGe islands driven by surface-mediated alloying [J].
Denker, U ;
Rastelli, A ;
Stoffel, M ;
Tersoff, J ;
Katsaros, G ;
Costantini, G ;
Kern, K ;
Jin-Phillipp, NY ;
Jesson, DE ;
Schmidt, OG .
PHYSICAL REVIEW LETTERS, 2005, 94 (21)
[8]   Influence of a thin GaAs cap layer on structural and optical properties of InAs quantum dots [J].
Ferdos, F ;
Wang, SM ;
Wei, YQ ;
Larsson, A ;
Sadeghi, M ;
Zhao, QX .
APPLIED PHYSICS LETTERS, 2002, 81 (07) :1195-1197
[9]   Intermixing and shape changes during the formation of InAs self-assembled quantum dots [J].
García, JM ;
MedeirosRibeiro, G ;
Schmidt, K ;
Ngo, T ;
Feng, JL ;
Lorke, A ;
Kotthaus, J ;
Petroff, PM .
APPLIED PHYSICS LETTERS, 1997, 71 (14) :2014-2016
[10]   Capping process of InAs/GaAs quantum dots studied by cross-sectional scanning tunneling microscopy [J].
Gong, Q ;
Offermans, P ;
Nötzel, R ;
Koenraad, PM ;
Wolter, JH .
APPLIED PHYSICS LETTERS, 2004, 85 (23) :5697-5699