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Nonlinear optical properties of graphene oxide in nanosecond and picosecond regimes
被引:342
作者:

Liu, Zhibo
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Nankai Univ, Minist Educ, Key Lab Weak Light Nonlinear Photon, Tianjin 300071, Peoples R China
Nankai Univ, Teda Appl Phys Sch, Tianjin 300071, Peoples R China Nankai Univ, Minist Educ, Key Lab Weak Light Nonlinear Photon, Tianjin 300071, Peoples R China

Wang, Yan
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机构:
Nankai Univ, Coll Chem, Key Lab Funct Polymer Mat, Tianjin 300071, Peoples R China
Nankai Univ, Coll Chem, Ctr Nanoscale Sci & Technol, Tianjin 300071, Peoples R China
Nankai Univ, Coll Chem, Inst Polymer Chem, Tianjin 300071, Peoples R China Nankai Univ, Minist Educ, Key Lab Weak Light Nonlinear Photon, Tianjin 300071, Peoples R China

Zhang, Xiaoliang
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机构:
Nankai Univ, Minist Educ, Key Lab Weak Light Nonlinear Photon, Tianjin 300071, Peoples R China
Nankai Univ, Teda Appl Phys Sch, Tianjin 300071, Peoples R China Nankai Univ, Minist Educ, Key Lab Weak Light Nonlinear Photon, Tianjin 300071, Peoples R China

Xu, Yanfei
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机构:
Nankai Univ, Coll Chem, Key Lab Funct Polymer Mat, Tianjin 300071, Peoples R China
Nankai Univ, Coll Chem, Ctr Nanoscale Sci & Technol, Tianjin 300071, Peoples R China
Nankai Univ, Coll Chem, Inst Polymer Chem, Tianjin 300071, Peoples R China Nankai Univ, Minist Educ, Key Lab Weak Light Nonlinear Photon, Tianjin 300071, Peoples R China

Chen, Yongsheng
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h-index: 0
机构:
Nankai Univ, Coll Chem, Key Lab Funct Polymer Mat, Tianjin 300071, Peoples R China
Nankai Univ, Coll Chem, Ctr Nanoscale Sci & Technol, Tianjin 300071, Peoples R China
Nankai Univ, Coll Chem, Inst Polymer Chem, Tianjin 300071, Peoples R China Nankai Univ, Minist Educ, Key Lab Weak Light Nonlinear Photon, Tianjin 300071, Peoples R China

Tian, Jianguo
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机构:
Nankai Univ, Minist Educ, Key Lab Weak Light Nonlinear Photon, Tianjin 300071, Peoples R China
Nankai Univ, Teda Appl Phys Sch, Tianjin 300071, Peoples R China Nankai Univ, Minist Educ, Key Lab Weak Light Nonlinear Photon, Tianjin 300071, Peoples R China
机构:
[1] Nankai Univ, Minist Educ, Key Lab Weak Light Nonlinear Photon, Tianjin 300071, Peoples R China
[2] Nankai Univ, Teda Appl Phys Sch, Tianjin 300071, Peoples R China
[3] Nankai Univ, Coll Chem, Key Lab Funct Polymer Mat, Tianjin 300071, Peoples R China
[4] Nankai Univ, Coll Chem, Ctr Nanoscale Sci & Technol, Tianjin 300071, Peoples R China
[5] Nankai Univ, Coll Chem, Inst Polymer Chem, Tianjin 300071, Peoples R China
基金:
高等学校博士学科点专项科研基金;
关键词:
absorption;
carbon nanotubes;
fullerenes;
nonlinear optics;
photon-photon interactions;
CARBON NANOTUBES;
ABSORPTION;
D O I:
10.1063/1.3068498
中图分类号:
O59 [应用物理学];
学科分类号:
摘要:
The nonlinear optical properties of graphene oxide (GO) were investigated at 532 nm in nanosecond and picosecond regimes. Results show that two-photon absorption dominates nonlinear absorption process of GO in the case of picosecond pulses, while excited state nonlinearities play an important role in the case of nanosecond pulses. Additionally, we compared nonlinear optical properties of three different dimensional carbon-based materials (two-dimensional graphene, one-dimensional carbon nanotube, and zero-dimensional fullerene) in nanosecond and picosecond regimes, respectively. The nonlinear mechanism of GO is distinctly different from nonlinear scattering of carbon nanotube and excited state nonlinearity of fullerene.
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