Nanostructure Engineering and Doping of Conjugated Carbon Nitride Semiconductors for Hydrogen Photosynthesis

被引：785

作者：

Lin, Zhenzhen ^{[1
,2
]}

Wang, Xinchen ^{[1
,2
]}

机构：

[1] Fuzhou Univ, Res Inst Photocatalysis, Fujian Prov Key Lab Photocatalysis, State Key Lab Breeding Base, Fuzhou 350002, Peoples R China

[2] Fuzhou Univ, Coll Chem & Chem Engn, Fuzhou 350002, Peoples R China

来源：

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION | 2013年 / 52卷 / 06期

基金：

中国国家自然科学基金;

关键词：

carbon nitride; conjugated polymers; doping; nanosheets; photosynthesis; FRUSTRATED LEWIS PAIRS; POLYMERS; BORON; ACTIVATION; EVOLUTION; OXIDATION; GRAPHENE;

D O I：

10.1002/anie.201209017

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Going flat out: Simultaneous modifications of the textural, surface, and electronic structures of a rigid conjugated carbon nitride polymer has been achieved using direct co-condensation of urea and Ph4BNa. This method gives boron-doped carbon nitride nanosheets (see picture) that optimize the capture of light, improve the charge-separation kinetics, and enhance the surface reactivity for hydrogen photosynthesis. Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

引用

页码：1735 / 1738

页数：4

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