Design criteria for transparent single-wall carbon nanotube thin-film transistors

被引:141
作者
Unalan, HE [1 ]
Fanchini, G [1 ]
Kanwal, A [1 ]
Du Pasquier, A [1 ]
Chhowalla, M [1 ]
机构
[1] Rutgers State Univ, Piscataway, NJ 08854 USA
关键词
D O I
10.1021/NL052406l
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A study based on two-dimensional percolation theory yielding quantitative parameters for optimum connectivity of transparent single-wall carbon nanotube (SWNT) thin films is reported. Optimum SWNT concentration in the filtrated solution was found to be 0.1 mg/L with a volume of 30 mL. Such parameters lead to SWNT fractions in the films of approximately Phi = 1.8 x 10(-3), much below the metallic percolation threshold, which is found to be similar to Phi(c) = 5.5 x 10(-3). Therefore, the performance of transparent carbon nanotube thin-film transistors is limited by the metallic SWNTs, even below their percolation threshold. We show how this effect is related to hopping or tunneling between neighboring metallic tubes.
引用
收藏
页码:677 / 682
页数:6
相关论文
共 16 条
[1]   Transparent and flexible carbon nanotube transistors [J].
Artukovic, E ;
Kaempgen, M ;
Hecht, DS ;
Roth, S ;
GrUner, G .
NANO LETTERS, 2005, 5 (04) :757-760
[2]   Logic circuits with carbon nanotube transistors [J].
Bachtold, A ;
Hadley, P ;
Nakanishi, T ;
Dekker, C .
SCIENCE, 2001, 294 (5545) :1317-1320
[3]   EXCLUDED VOLUME AND ITS RELATION TO THE ONSET OF PERCOLATION [J].
BALBERG, I ;
ANDERSON, CH ;
ALEXANDER, S ;
WAGNER, N .
PHYSICAL REVIEW B, 1984, 30 (07) :3933-3943
[4]   ALIGNED CARBON NANOTUBE FILMS - PRODUCTION AND OPTICAL AND ELECTRONIC-PROPERTIES [J].
DEHEER, WA ;
BACSA, WS ;
CHATELAIN, A ;
GERFIN, T ;
HUMPHREYBAKER, R ;
FORRO, L ;
UGARTE, D .
SCIENCE, 1995, 268 (5212) :845-847
[5]  
Dresselhaus MS, 2001, CARBON NANOTUBES SYN
[6]   Percolation in transparent and conducting carbon nanotube networks [J].
Hu, L ;
Hecht, DS ;
Grüner, G .
NANO LETTERS, 2004, 4 (12) :2513-2517
[7]   Electronic devices based on purified carbon nanotubes grown by high-pressure decomposition of carbon monoxide [J].
Johnston, DE ;
Islam, MF ;
Yodh, AG ;
Johnson, AT .
NATURE MATERIALS, 2005, 4 (08) :589-592
[8]   Single- and multi-wall carbon nanotube field-effect transistors [J].
Martel, R ;
Schmidt, T ;
Shea, HR ;
Hertel, T ;
Avouris, P .
APPLIED PHYSICS LETTERS, 1998, 73 (17) :2447-2449
[9]  
Mott N.F., 1979, ELECT PROCESSES NONC, V2nd ed., P33
[10]   Conducting and transparent single-wall carbon nanotube electrodes for polymer-fullerene solar cells [J].
Pasquier, AD ;
Unalan, HE ;
Kanwal, A ;
Miller, S ;
Chhowalla, M .
APPLIED PHYSICS LETTERS, 2005, 87 (20) :1-3