Growth interruption to tune the emission of InAs quantum dots embedded in InGaAs matrix in the long wavelength region

被引:38
作者
Convertino, A [1 ]
Cerri, L [1 ]
Leo, G [1 ]
Viticoli, S [1 ]
机构
[1] CNR, Ist Studio Mat Nanostrutturati, I-00016 Monterotondo, Italy
关键词
surface processes; molecular beam epitaxy; nanomaterials;
D O I
10.1016/j.jcrysgro.2003.09.034
中图分类号
O7 [晶体学];
学科分类号
0702 ; 070205 ; 0703 ; 080501 ;
摘要
We investigate the effects of combining growth interruption (GI) and InGaAs strain reducing matrix at low In content on the optical properties of Stanski-Krastanow InAs QDs grown by molecular beam epitaxy. Atomic force microscopy and Photoluminescence (PL) measurements were carried out on three series of uncapped and capped samples grown in different conditions: (a) low arsenic pressure (As BEP = 4 x 10(-6) Torr) and relatively low InAs growth temperature (T-InAs = 530degreesC); (b) low As BEP (4 x 10(-6) Torr) and high T-InAs (545degreesC); (c) high As BEP (7 x 10(-6) Torr) and low T-InAs (530degreesC). Our studies clearly show that in the three growth regimes, GI causes very different effects on the morphological and optical properties of InAs QDs embedded in InGaAs matrix (In=0.12), ruled by the In diffusion and desorption processes. In particular, for samples grown at 530degreesC and As BeP = 4 x 10(-6) Torr (series a), the arrangment of GI and QD embedding in an InGaAs matrix at low In content is an effcient method to tune the InAs QD PL emission and to improve their optical quality. In this case, indeed, the increase of the interruption time up to 300 s introduces a strong redshift (similar to 110 meV) in the PL peak with a decreasing of the linewidths from 52 to 26 meV obtaining room temperature emission characterized by a narrow peak close to 1.3 mum. (C) 2003 Elsevier B.V. All rights reserved.
引用
收藏
页码:458 / 465
页数:8
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