Surface-related emission in highly luminescent CdSe quantum dots

被引:497
作者
Wang, XY
Qu, LH
Zhang, JY
Peng, XG
Xiao, M [1 ]
机构
[1] Univ Arkansas, Dept Phys, Fayetteville, AR 72701 USA
[2] Univ Arkansas, Dept Chem & Biochem, Fayetteville, AR 72701 USA
关键词
D O I
10.1021/nl0342491
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
We report our experimental studies of surface-related emission in highly luminescent CdSe quantum dots (QDs) with controlled quantum yield and photooxidation by time-resolved photoluminescence measurements. This kind of surface-related emission, with a radiative lifetime of tens of nanoseconds, implies the involvement of surface states in the carrier recombination process of such highly luminescent CdSe QDs.
引用
收藏
页码:1103 / 1106
页数:4
相关论文
共 28 条
[1]   Semiconductor clusters, nanocrystals, and quantum dots [J].
Alivisatos, AP .
SCIENCE, 1996, 271 (5251) :933-937
[2]   LUMINESCENCE PROPERTIES OF CDSE QUANTUM CRYSTALLITES - RESONANCE BETWEEN INTERIOR AND SURFACE LOCALIZED STATES [J].
BAWENDI, MG ;
CARROLL, PJ ;
WILSON, WL ;
BRUS, LE .
JOURNAL OF CHEMICAL PHYSICS, 1992, 96 (02) :946-954
[3]   QUANTUM CRYSTALLITES AND NONLINEAR OPTICS [J].
BRUS, L .
APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING, 1991, 53 (06) :465-474
[4]   DIRECT DETERMINATION OF III-V SEMICONDUCTOR SURFACE BAND-GAPS [J].
CARSTENSEN, H ;
CLAESSEN, R ;
MANZKE, R ;
SKIBOWSKI, M .
PHYSICAL REVIEW B, 1990, 41 (14) :9880-9885
[5]   Surface structure of cadmium selenide nanocrystallites [J].
Carter, AC ;
Bouldin, CE ;
Kemner, KM ;
Bell, MI ;
Woicik, JC ;
Majetich, SA .
PHYSICAL REVIEW B, 1997, 55 (20) :13822-13828
[6]   Polarization spectroscopy of single CdSe quantum rods [J].
Chen, X ;
Nazzal, A ;
Goorskey, D ;
Xiao, M ;
Peng, ZA ;
Peng, XG .
PHYSICAL REVIEW B, 2001, 64 (24) :2453041-2453044
[7]   Time-gated biological imaging by use of colloidal quantum dots [J].
Dahan, M ;
Laurence, T ;
Pinaud, F ;
Chemla, DS ;
Alivisatos, AP ;
Sauer, M ;
Weiss, S .
OPTICS LETTERS, 2001, 26 (11) :825-827
[8]   InP quantum dots: Electronic structure, surface effects, and the redshifted emission [J].
Fu, HX ;
Zunger, A .
PHYSICAL REVIEW B, 1997, 56 (03) :1496-1508
[9]   Electron and hole relaxation pathways in semiconductor quantum dots [J].
Klimov, VI ;
McBranch, DW ;
Leatherdale, CA ;
Bawendi, MG .
PHYSICAL REVIEW B, 1999, 60 (19) :13740-13749
[10]   Dominant role of surface states in photoexcited carrier dynamics in CdSe nanocrystalline films prepared by chemical deposition [J].
Maly, P ;
Kudrna, J ;
Trojánek, F ;
Mikes, D ;
Nemec, P ;
Maciel, AC ;
Ryan, JF .
APPLIED PHYSICS LETTERS, 2000, 77 (15) :2352-2354