Electronic structure of Y2-xCaxBaNiO5 from photoemission and inverse photoemission

被引:29
作者
Maiti, K [1 ]
Sarma, DD
机构
[1] Indian Inst Sci, Solid State & Struct Chem Unit, Bangalore 560012, Karnataka, India
[2] Indian Inst Sci, Jawaharlal Nehru Ctr Adv Sci Res, Bangalore 560012, Karnataka, India
来源
PHYSICAL REVIEW B | 1998年 / 58卷 / 15期
关键词
D O I
10.1103/PhysRevB.58.9746
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We investigate the electronic structure of a one-dimensional spin-1 system, Y2BaNiO5, and hole-doped Y2-xCaxBaNiO5 for x=0.2 and 0.4, employing photoemission and inverse photoemission spectroscopies. Y2BaNiO5 has a charge excitation gap of about 2.3 eV. Hole doping via Ca substitution in this system introduces new localized states within this gap. The existence of a finite gap (similar to 0.6 eV), even in doped compounds with a variable-range-hopping transport, indicates the importance of correlation effects and disorder in determining the electronic structure in this system. [S0163-1829(98)01739-1].
引用
收藏
页码:9746 / 9751
页数:6
相关论文
共 46 条
[31]   Electronic structure of La1-xSrxCrO3 [J].
Maiti, K ;
Sarma, DD .
PHYSICAL REVIEW B, 1996, 54 (11) :7816-7822
[32]  
MAITI K, UNPUB
[33]   Raman-scattering evidence for free spinons in the one-dimensional spin-1/2 chains of Sr2CuO3 and SrCuO2 [J].
Misochko, OV ;
Tajima, S ;
Urano, C ;
Eisaki, H ;
Uchida, S .
PHYSICAL REVIEW B, 1996, 53 (22) :14733-14736
[34]   TEMPERATURE-DEPENDENCE OF THE ELECTRON-SPIN-RESONANCE SPECTRUM OF THE CHAIN-END S = 1/2 MODES IN AN S = 1 ANTIFERROMAGNETIC CHAIN [J].
MITRA, PP ;
HALPERIN, BI ;
AFFLECK, I .
PHYSICAL REVIEW B, 1992, 45 (10) :5299-5306
[35]   Magnetic susceptibility of ideal spin 1/2 Heisenberg antiferromagnetic chain systems, Sr2CuO3 and SrCuO2 [J].
Motoyama, N ;
Eisaki, H ;
Uchida, S .
PHYSICAL REVIEW LETTERS, 1996, 76 (17) :3212-3215
[36]   O 1s near-edge x-ray absorption of La2-xSrxNiO4+delta: Holes, polarons, and excitons [J].
Pellegrin, E ;
Zaanen, J ;
Lin, HJ ;
Meigs, G ;
Chen, CT ;
Ho, GH ;
Eisaki, H ;
Uchida, S .
PHYSICAL REVIEW B, 1996, 53 (16) :10667-10679
[37]   SPECIFIC-HEAT OF DEFECTS IN HALDANE SYSTEMS Y2BANIO5 AND NENP - ABSENCE OF FREE SPIN-1/2 EXCITATIONS [J].
RAMIREZ, AP ;
CHEONG, SW ;
KAPLAN, ML .
PHYSICAL REVIEW LETTERS, 1994, 72 (19) :3108-3111
[38]   BAND THEORY FOR GROUND-STATE PROPERTIES AND EXCITATION-SPECTRA OF PEROVSKITE LAMO(3) (M=MN, FE, CO, NI) [J].
SARMA, DD ;
SHANTHI, N ;
BARMAN, SR ;
HAMADA, N ;
SAWADA, H ;
TERAKURA, K .
PHYSICAL REVIEW LETTERS, 1995, 75 (06) :1126-1129
[39]   APPEARANCE OF CORRELATION-EFFECTS IN U INTERMETALLICS [J].
SARMA, DD ;
HILLEBRECHT, FU ;
SPEIER, W ;
MARTENSSON, N ;
KOELLING, DD .
PHYSICAL REVIEW LETTERS, 1986, 57 (17) :2215-2218
[40]   PHOTOEMISSION AND INVERSE PHOTOEMISSION OF TRANSITION-METAL SILICIDES [J].
SPEIER, W ;
VONLEUKEN, E ;
FUGGLE, JC ;
SARMA, DD ;
KUMAR, L ;
DAUTH, B ;
BUSCHOW, KHJ .
PHYSICAL REVIEW B, 1989, 39 (09) :6008-6016