Organic Field-Effect Transistors based on Highly Ordered Single Polymer Fibers

被引：218

作者：

Wang, Suhao ^{[1
]}

Kappl, Michael ^{[1
]}

Liebewirth, Ingo ^{[1
]}

Mueller, Maren ^{[1
]}

Kirchhoff, Katrin ^{[1
]}

Pisula, Wojciech ^{[1
]}

Muellen, Klaus ^{[1
]}

机构：

[1] Max Planck Inst Polymer Res, D-55128 Mainz, Germany

来源：

ADVANCED MATERIALS | 2012年 / 24卷 / 03期

关键词：

conjugated donor-acceptor copolymer; single polymer fibers; organic electronics; field-effect transistors; self-assembly; THIN-FILM TRANSISTORS; HIGH-PERFORMANCE; SEMICONDUCTING POLYMERS; CHARGE-TRANSPORT; COPOLYMERS; RIBBONS; SURFACE;

D O I：

10.1002/adma.201103057

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Ultrahigh-mobility organic field-effect transistors (OFETs) based on a CDT-BTZ donor-acceptor copolymer are realized by reaching high molecular order and pronounced alignment in single fibers within a short OFET channel via solution processing. The macromolecules directionally self-assemble in a quasi crystal-like order in the fibers providing in this way an unhindered charge carrier pathway with mobilities as high as 5.5 cm(2) V-1 s(-1).

引用

收藏

页码：417 / +

页数：5

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[11] Single-crystal polythiophene microwires grown by self-assembly [J].

Kim, DH ;

Han, JT ;

Park, YD ;

Jang, Y ;

Cho, JH ;

Hwang, M ;

Cho, K .

ADVANCED MATERIALS, 2006, 18 (06) :719-+

[12] Polyindolo[3,2-b]carbazoles:: A new class of p-channel semiconductor polymers for organic thin-film transistors [J].

Li, Yuning ;

Wu, Yiliang ;

Ong, Beng S. .

MACROMOLECULES, 2006, 39 (19) :6521-6527

[13] Poly(2,5-bis(2-thienyl)-3,6-dialkylthieno[3,2-b]thiophene)s-high-mobility semiconductors for thin-film transistors [J].

Li, Yuning ;

Wu, Yiliang ;

Liu, Ping ;

Birau, Maria ;

Pan, Hualong ;

Ong, Beng S. .

ADVANCED MATERIALS, 2006, 18 (22) :3029-+

[14] Solution-Processable Organic Single Crystals with Bandlike Transport in Field-Effect Transistors [J].

Liu, Chuan ;

Minari, Takeo ;

Lu, Xubing ;

Kumatani, Akichika ;

Takimiya, Kazuo ;

Tsukagoshi, Kazuhito .

ADVANCED MATERIALS, 2011, 23 (04) :523-+

[15] Controlling Poly(3-hexylthiophene) Crystal Dimension: Nanowhiskers and Nanoribbons [J].

Liu, Jianhua ;

Arif, Mohammad ;

Zou, Jianhua ;

Khondaker, Saiful I. ;

Zhai, Lei .

MACROMOLECULES, 2009, 42 (24) :9390-9393

[16] Highly disordered polymer field effect transistors:: N-alkyl dithieno[3,2-b:2′,3′-d]pyrrole-based copolymers with surprisingly high charge carrier mobilities [J].

Liu, Junying ;

Zhang, Rui ;

Sauve, Genevieve ;

Kowalewski, Tomasz ;

McCullough, Richard D. .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2008, 130 (39) :13167-13176

[17] Highly Efficient Patterning of Organic Single-Crystal Transistors from the Solution Phase [J].

Mannsfeld, Stefan C. B. ;

Sharei, Armon ;

Liu, Shuhong ;

Roberts, Mark E. ;

McCulloch, Iain ;

Heeney, Martin ;

Bao, Zhenan .

ADVANCED MATERIALS, 2008, 20 (21) :4044-+

[18] Liquid-crystalline semiconducting polymers with high charge-carrier mobility [J].

Mcculloch, I ;

Heeney, M ;

Bailey, C ;

Genevicius, K ;

Macdonald, I ;

Shkunov, M ;

Sparrowe, D ;

Tierney, S ;

Wagner, R ;

Zhang, WM ;

Chabinyc, ML ;

Kline, RJ ;

Mcgehee, MD ;

Toney, MF .

NATURE MATERIALS, 2006, 5 (04) :328-333

[19] Solution-processed, high-performance n-channel organic microwire transistors [J].

Oh, Joon Hak ;

Lee, Hang Woo ;

Mannsfeld, Stefan ;

Stoltenberg, Randall M. ;

Jung, Eric ;

Jin, Yong Wan ;

Kim, Jong Min ;

Yoo, Ji-Beom ;

Bao, Zhenan .

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2009, 106 (15) :6065-6070

[20] Novel thiophene-thiazolothiazole copolymers for organic field-effect transistors [J].

Osaka, Itaru ;

Sauve, Genevieve ;

Zhang, Rui ;

Kowalewski, Tomasz ;

McCullough, Richard D. .

ADVANCED MATERIALS, 2007, 19 (23) :4160-+

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