Interplay of thermal and quantum spin fluctuations in the kagome lattice compound herbertsmithite

被引:93
作者
Wulferding, Dirk [1 ]
Lemmens, Peter [1 ]
Scheib, Patric [1 ]
Roeder, Jens [2 ]
Mendels, Philippe [3 ]
Chu, Shaoyan [4 ]
Han, Tianheng [5 ]
Lee, Young S. [5 ]
机构
[1] Tech Univ Carolo Wilhelmina Braunschweig, Inst Condensed Matter Phys, D-38106 Braunschweig, Germany
[2] Tech Univ Carolo Wilhelmina Braunschweig, Inst Phys & Theoret Chem, D-38106 Braunschweig, Germany
[3] Univ Paris 11, CNRS, Phys Solides Lab, UMR 8502, F-91405 Orsay, France
[4] MIT, Ctr Mat Sci & Engn, Cambridge, MA 02139 USA
[5] MIT, Dept Condensed Matter Phys, Cambridge, MA 02139 USA
来源
PHYSICAL REVIEW B | 2010年 / 82卷 / 14期
关键词
ANTIFERROMAGNET; ORDER;
D O I
10.1103/PhysRevB.82.144412
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We present a Raman spectroscopic investigation of the herbertsmithite ZnCu3(OH)(6)Cl-2, a realization of a Heisenberg s=1/2 antiferromagnet on a perfect kagome lattice. Focusing on its magnetic excitation spectrum we find two components, a high-temperature quasielastic signal and a low temperature, broad maximum. The latter has a linear low-energy slope and extends to high energy. We have investigated the temperature dependence and symmetry properties of both signals. Our data agree with previous calculations and point to a gapless spin liquid ground state.
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页数:6
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