Low Temperature Raman Study of the Electron Coherence Length near Graphene Edges

被引:70
作者
Beams, Ryan [1 ]
Cancado, Luiz Gustavo [2 ]
Novotny, Lukas [1 ]
机构
[1] Univ Rochester, Inst Opt, Rochester, NY 14627 USA
[2] Univ Fed Minas Gerais, Dept Fis, BR-30123970 Belo Horizonte, MG, Brazil
关键词
Graphene; optical properties; Raman scattering; spectroscopy; defects; localization; SCATTERING;
D O I
10.1021/nl104134a
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
We developed a novel optical defocusing method for studying spatial coherence of photoexcited electrons and holes near edges of graphene. Our method is applied to measure the localization l(D) of the disorder-induced Raman D band (similar to 1350 cm(-1)) with a resolution of a few nanometers. Raman scattering experiments performed in a helium bath cryostat reveal that as temperature is decreased from 300 to 1.55 K, the length l(D) increases. We found that the localization of the D band varies as 1/T-1/2, giving strong evidence that l(D) scales with the coherence length of photoexcited electrons near graphene edges.
引用
收藏
页码:1177 / 1181
页数:5
相关论文
共 29 条
[1]   Ballistic transport in graphene nanostrips in the presence of disorder: Importance of edge effects [J].
Areshkin, Denis A. ;
Gunlycke, Daniel ;
White, Carter T. .
NANO LETTERS, 2007, 7 (01) :204-210
[2]   Carbon-based electronics [J].
Avouris, Phaedon ;
Chen, Zhihong ;
Perebeinos, Vasili .
NATURE NANOTECHNOLOGY, 2007, 2 (10) :605-615
[3]   Interplay of Coulomb and electron-phonon interactions in graphene [J].
Basko, D. M. ;
Aleiner, I. L. .
PHYSICAL REVIEW B, 2008, 77 (04)
[4]  
BEENAKKER CWJ, 1991, SOLID STATE PHYS, V44, P1
[5]   Influence of the atomic structure on the Raman spectra of graphite edges -: art. no. 247401 [J].
Cançado, LG ;
Pimenta, MA ;
Neves, BRA ;
Dantas, MSS ;
Jorio, A .
PHYSICAL REVIEW LETTERS, 2004, 93 (24)
[6]   Raman Spectroscopy of Graphene Edges [J].
Casiraghi, C. ;
Hartschuh, A. ;
Qian, H. ;
Piscanec, S. ;
Georgi, C. ;
Fasoli, A. ;
Novoselov, K. S. ;
Basko, D. M. ;
Ferrari, A. C. .
NANO LETTERS, 2009, 9 (04) :1433-1441
[7]   The carbon new age [J].
Castro Neto, Antonio H. .
MATERIALS TODAY, 2010, 13 (03) :12-17
[8]   Graphene nano-ribbon electronics [J].
Chen, Zhihong ;
Lin, Yu-Ming ;
Rooks, Michael J. ;
Avouris, Phaedon .
PHYSICA E-LOW-DIMENSIONAL SYSTEMS & NANOSTRUCTURES, 2007, 40 (02) :228-232
[9]   Electronic properties and quantum transport in Graphene-based nanostructures [J].
Dubois, S. M. -M. ;
Zanolli, Z. ;
Declerck, X. ;
Charlier, J. -C. .
EUROPEAN PHYSICAL JOURNAL B, 2009, 72 (01) :1-24
[10]   Raman spectrum of graphene and graphene layers [J].
Ferrari, A. C. ;
Meyer, J. C. ;
Scardaci, V. ;
Casiraghi, C. ;
Lazzeri, M. ;
Mauri, F. ;
Piscanec, S. ;
Jiang, D. ;
Novoselov, K. S. ;
Roth, S. ;
Geim, A. K. .
PHYSICAL REVIEW LETTERS, 2006, 97 (18)