Recent Advances in Conjugated Polyelectrolytes for Emerging Optoelectronic Applications

被引：326

作者：

Duarte, Aidee ^{[2
]}

Pu, Kan-Yi ^{[1
]}

Liu, Bin ^{[1
]}

Bazan, Guillermo C. ^{[2
,3
]}

机构：

[1] Natl Univ Singapore, Dept Chem & Biomol Engn, Singapore 117576, Singapore

[2] Univ Calif Santa Barbara, Dept Chem & Biochem, Ctr Polymers & Organ Solids, Santa Barbara, CA 93106 USA

[3] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA

来源：

CHEMISTRY OF MATERIALS | 2011年 / 23卷 / 03期

基金：

美国国家科学基金会;

关键词：

POLYHEDRAL OLIGOMERIC SILSESQUIOXANE; RESONANCE ENERGY-TRANSFER; TIME FLUORESCENCE ASSAY; INTERPOLYELECTROLYTE COMPLEXES; SOLAR-CELLS; NONSPECIFIC INTERACTIONS; DNA DETECTION; LABEL-FREE; POLY(P-PHENYLENE ETHYNYLENE); OPTICAL AMPLIFICATION;

D O I：

10.1021/cm102196t

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

This review summarizes recent advances in the science and applications of conjugated polyelectrolytes (CPEs), with an emphasis on direct visual sensing, cellular imaging, and the fabrication of optoelectronic devices. CPEs backbones that incorporate donor-acceptor units are useful for direct visual sensing, whereas CPEs with hyperbranched structures, or biocompatible long side chains, are particularly useful for cellular imaging. With specially designed counterions, CPEs also demonstrate unique function in device fabrication and operation, for example, in dye-sensitized solar cells (DSSCs), bulk heterojunction (BHJ) solar cells, polymer light-emitting diodes (PLEDs), polymer light-emitting electrochemical cells (PLECs), and organic thin film transistors (OFET). Additionally, new strategies to modify and optimize CPE properties for specific applications are provided. The work summarized herein not only illustrates relationships between molecular structures and function, but also highlights how the structural versatility of CPEs makes them a unique category of multifunctional materials with the potential for fulfilling a variety of optical and electronic applications in solution, mixed media, and in the solid state.

引用

页码：501 / 515

页数：15

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