Charge Transport Orthogonality in All-Polymer Blend Transistors, Diodes, and Solar Cells

被引:61
作者
Fabiano, Simone [1 ]
Himmelberger, Scott [2 ]
Drees, Martin [3 ]
Chen, Zhihua [3 ]
Altamimi, Rashid M. [4 ]
Salleo, Alberto [2 ]
Loi, Maria Antonietta [1 ]
Facchetti, Antonio [3 ]
机构
[1] Univ Groningen, Zernike Inst Adv Mat, NL-9747 AG Groningen, Netherlands
[2] Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA
[3] Polyera Corp, Skokie, IL 60077 USA
[4] King Abdulaziz City Sci & Technol, Petrochem Res Inst, Riyadh 11442, Saudi Arabia
基金
美国国家科学基金会;
关键词
all-polymer blends; charge transport; field-effect transistors; hierarchical structures; organic solar cells; FIELD-EFFECT TRANSISTORS; THIN-FILMS; POLY(3-HEXYLTHIOPHENE); AMBIPOLAR; PERFORMANCE; COPOLYMER; CRYSTALLIZATION; AGGREGATION; SEPARATION; TEXTURE;
D O I
10.1002/aenm.201301409
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Polymer aggregation and phase separation of polymer-polymer blends are effectively tuned from self-stratified to laterally phase-separated by adjusting the relative solubility of the two polymers in the mixture. This is found to dramatically alter the charge transport characteristics from a preferential in-plane to an out-of-plane direction, revealing the critical dependence of the resulting device performance on the film morphology and structure of the active layer. © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
引用
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页数:7
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