Observation of optical gain in solutions of CdS quantum dots at room temperature in the blue region

被引:21
作者
Darugar, Qusai [1 ]
Qian, Wei [1 ]
El-Sayed, Mostafa A. [1 ]
机构
[1] Georgia Inst Technol, Sch Chem & Biochem, Laser Dynam Lab, Atlanta, GA 30332 USA
基金
美国国家科学基金会;
关键词
D O I
10.1063/1.2217138
中图分类号
O59 [应用物理学];
学科分类号
摘要
The optical gain dynamics has been studied for two CdS quantum dot samples dispersed in toluene at room temperature. This was carried out by using femtosecond transient absorption technique with an excitation at 400 nm and gain measurement was studied at the fluorescence maxima (440 and 460 nm). The optical gain lifetime was found to be as long as 20 ps under pump fluence as low as 0.77 mJ/cm(2). The low threshold is the result of long lifetime of electrons and holes and narrow emission bandwidth. These results suggest that CdS quantum dots in solution are excellent gain media for optically pumped high power blue lasers.
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页数:3
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共 28 条
[1]   Semiconductor clusters, nanocrystals, and quantum dots [J].
Alivisatos, AP .
SCIENCE, 1996, 271 (5251) :933-937
[2]   MULTIDIMENSIONAL QUANTUM WELL LASER AND TEMPERATURE-DEPENDENCE OF ITS THRESHOLD CURRENT [J].
ARAKAWA, Y ;
SAKAKI, H .
APPLIED PHYSICS LETTERS, 1982, 40 (11) :939-941
[3]   GAIN AND THE THRESHOLD OF 3-DIMENSIONAL QUANTUM-BOX LASERS [J].
ASADA, M ;
MIYAMOTO, Y ;
SUEMATSU, Y .
IEEE JOURNAL OF QUANTUM ELECTRONICS, 1986, 22 (09) :1915-1921
[4]   QUASI-CONTINUOUS GAIN IN SOL-GEL DERIVED CDS QUANTUM DOTS [J].
BUTTY, J ;
HU, YZ ;
PEYGHAMBARIAN, N ;
KAO, YH ;
MACKENZIE, JD .
APPLIED PHYSICS LETTERS, 1995, 67 (18) :2672-2674
[5]   Blue semiconductor nanocrystal laser [J].
Chan, Y ;
Steckel, JS ;
Snee, PT ;
Caruge, JM ;
Hodgkiss, JM ;
Nocera, DG ;
Bawendi, MG .
APPLIED PHYSICS LETTERS, 2005, 86 (07) :1-3
[6]   Multiexcitonic two-state lasing in a CdSe nanocrystal laser [J].
Chan, Y ;
Caruge, JM ;
Snee, PT ;
Bawendi, MG .
APPLIED PHYSICS LETTERS, 2004, 85 (13) :2460-2462
[7]   Optical gain from InAs nanocrystal quantum dots in a polymer matrix [J].
Chen, G ;
Rapaport, R ;
Fuchs, DT ;
Lucas, L ;
Lovinger, AJ ;
Vilan, S ;
Aharoni, A ;
Banin, U .
APPLIED PHYSICS LETTERS, 2005, 87 (25) :1-3
[8]   Spectrally resolved dynamics of energy transfer in quantum-dot assemblies: Towards engineered energy flows in artificial materials [J].
Crooker, SA ;
Hollingsworth, JA ;
Tretiak, S ;
Klimov, VI .
PHYSICAL REVIEW LETTERS, 2002, 89 (18)
[9]   The electronic structure of semiconductor nanocrystals [J].
Efros, AL ;
Rosen, M .
ANNUAL REVIEW OF MATERIALS SCIENCE, 2000, 30 :475-521
[10]   Microscopic theory of optical gain in small semiconductor quantum dots [J].
Hu, YZ ;
Giessen, H ;
Peyghambarian, N ;
Koch, SW .
PHYSICAL REVIEW B, 1996, 53 (08) :4814-4822