Development of n-type organic semiconductors for thin film transistors: a viewpoint of molecular design

被引:244
作者
Gao, Xike [1 ]
Hu, Yunbin [1 ]
机构
[1] Chinese Acad Sci, Shanghai Inst Organ Chem, Mat Sci Lab, Shanghai 200032, Peoples R China
关键词
FIELD-EFFECT TRANSISTORS; HIGH-ELECTRON-MOBILITY; EXPANDED NAPHTHALENE DIIMIDES; ONE-POT SYNTHESIS; HIGH-PERFORMANCE; CHANNEL TRANSISTOR; POLYMER SEMICONDUCTORS; PERYLENE DIIMIDE; COMPLEMENTARY CIRCUITS; CONJUGATED COPOLYMER;
D O I
10.1039/c3tc32046d
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The past ten years have witnessed great progress of n-type organic semiconductors (OSCs) for organic thin film transistors (OTFTs), while the device performance and ambient stability of n-type OSCs are still outmatched by their p-type counterparts. The pursuit of high-performance ambient-stable n-type OSCs for OTFTs is highly desirable for realizing robust, large-area and low-cost organic integrated circuits. In this feature article, we'll review the development of n-type OSCs for OTFTs from a viewpoint of molecular design, where more than nine molecular design strategies with >120 representative n-type OSCs are summarized and analyzed to give some valuable insights for this significant but challenging field.
引用
收藏
页码:3099 / 3117
页数:19
相关论文
共 170 条
[61]   Air-Stable n-Type Organic Field-Effect Transistors Based on 4,9-Dihydro-s-indaceno[1,2-b:5,6-b′]dithiazole-4,9-dione Unit [J].
Ie, Yutaka ;
Ueta, Masashi ;
Nitani, Masashi ;
Tohnai, Norimitsu ;
Miyata, Mikiji ;
Tada, Hirokazu ;
Aso, Yoshio .
CHEMISTRY OF MATERIALS, 2012, 24 (16) :3285-3293
[62]   Phthalocyanines - Versatile components of molecular conductors [J].
Inabe, T ;
Tajima, H .
CHEMICAL REVIEWS, 2004, 104 (11) :5503-5533
[63]   High mobility n-channel single-crystal field-effect transistors based on 5,7,12,14-tetrachloro-6,13-diazapentacene [J].
Islam, Md Minarul ;
Pola, Someshwar ;
Tao, Yu-Tai .
CHEMICAL COMMUNICATIONS, 2011, 47 (22) :6356-6358
[64]   High-mobility air-stable n-type semiconductors with processing versatility:: Dicyanoperylene-3,4:9,10-bis(dicarboximides) [J].
Jones, BA ;
Ahrens, MJ ;
Yoon, MH ;
Facchetti, A ;
Marks, TJ ;
Wasielewski, MR .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2004, 43 (46) :6363-6366
[65]   Tuning orbital energetics in arylene diimide semiconductors. Materials design for ambient stability of n-type charge transport [J].
Jones, Brooks A. ;
Facchetti, Antonio ;
Wasielewski, Michael R. ;
Marks, Tobin J. .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2007, 129 (49) :15259-15278
[66]   Cyanonaphthalene diimide semiconductors for air-stable, flexible, and optically transparent n-channel field-effect transistors [J].
Jones, Brooks A. ;
Facchetti, Antonio ;
Marks, Tobin J. ;
Wasielewski, Michael R. .
CHEMISTRY OF MATERIALS, 2007, 19 (11) :2703-2705
[67]   Molecular Design and Synthetic Approaches to Electron-Transporting Organic Transistor Semiconductors [J].
Jung, Byung Jun ;
Tremblay, Noah J. ;
Yeh, Ming-Ling ;
Katz, Howard E. .
CHEMISTRY OF MATERIALS, 2011, 23 (03) :568-582
[68]   Air-Operable, High-Mobility Organic Transistors with Semifluorinated Side Chains and Unsubstituted Naphthalenetetracarboxylic Diimide Cores: High Mobility and Environmental and Bias Stress Stability from the Perfluorooctylpropyl Side Chain [J].
Jung, Byung Jun ;
Lee, Kyusang ;
Sun, Jia ;
Andreou, Andreas G. ;
Katz, Howard E. .
ADVANCED FUNCTIONAL MATERIALS, 2010, 20 (17) :2930-2944
[69]   Low-Temperature-Processible, Transparent, and Air-Operable n-Channel Fluorinated Phenylethylated Naphthalenetetracarboxylic Diimide Semiconductors Applied to Flexible Transistors [J].
Jung, Byung Jun ;
Sun, Jia ;
Lee, Taegweon ;
Sarjeant, Amy ;
Katz, Howard E. .
CHEMISTRY OF MATERIALS, 2009, 21 (01) :94-101
[70]   A thermally resistant and air-stable n-type organic semiconductor: Naphthalene diimide of 3,5-bis-trifluoromethyl aniline [J].
Jung, Yunoh ;
Baeg, Kang-Jun ;
Kim, Dong-Yu ;
Someya, Takao ;
Park, Soo Young .
SYNTHETIC METALS, 2009, 159 (19-20) :2117-2121