Discrimination of Nuclear Explosions against Civilian Sources Based on Atmospheric Xenon Isotopic Activity Ratios

被引:142
作者
Kalinowski, Martin B. [1 ]
Axelsson, Anders [2 ]
Bean, Marc [3 ]
Blanchard, Xavier [4 ]
Bowyer, Theodore W. [5 ]
Brachet, Guy [4 ]
Hebel, Simon [1 ]
McIntyre, Justin I. [4 ]
Peters, Jana [1 ]
Pistner, Christoph [6 ]
Raith, Maria [7 ]
Ringbom, Anders [8 ]
Saey, Paul R. J. [9 ]
Schlosser, Clemens [10 ]
Stocki, Trevor J. [3 ]
Taffary, Thomas [4 ]
Ungar, R. Kurt [3 ]
机构
[1] Carl Friedrich von Weizsacker Ctr Sci & Peace Res, D-20144 Hamburg, Germany
[2] IAEA, A-1400 Vienna, Austria
[3] Radiat Protect Bur, Ottawa, ON K1A 1C1, Canada
[4] CEA, DAM, DIF, F-91297 Arpajon, France
[5] Pacific NW Natl Lab, Richland, WA 99352 USA
[6] Oko Inst eV, D-64295 Darmstadt, Germany
[7] Seibersdorf Res GmbH, Austrian Res Ctr, A-2444 Seibersdorf, Austria
[8] Swedish Def Res Agcy FOI, S-17290 Stockholm, Sweden
[9] Vienna Int Ctr, Provis Tech Secretariat, Preparatory Commiss, Comprehens Nucl Test Ban Treaty Org CTBTO, A-1400 Vienna, Austria
[10] Fed Off Radiat Protect BfS, D-79098 Freiburg, Germany
关键词
CTBT; environmental monitoring; international monitoring system; isotope activity ratios; noble gas; radioactivity monitoring; radioxenon; source discrimination; test ban; xenon; TEST-BAN TREATY;
D O I
10.1007/s00024-009-0032-1
中图分类号
P3 [地球物理学]; P59 [地球化学];
学科分类号
0708 ; 070902 ;
摘要
A global monitoring system for atmospheric xenon radioactivity is being established as part of the International Monitoring System that will verify compliance with the Comprehensive Nuclear-Test-Ban Treaty (CTBT) once the treaty has entered into force. This paper studies isotopic activity ratios to support the interpretation of observed atmospheric concentrations of Xe-135, Xe-133m, Xe-133 and Xe-131m. The goal is to distinguish nuclear explosion sources from civilian releases. Simulations of nuclear explosions and reactors, empirical data for both test and reactor releases as well as observations by measurement stations of the International Noble Gas Experiment (INGE) are used to provide a proof of concept for the isotopic ratio based method for source discrimination.
引用
收藏
页码:517 / 539
页数:23
相关论文
共 34 条
[21]   SAUNA - a system for automatic sampling, processing, and analysis of radioactive xenon [J].
Ringbom, A ;
Larson, T ;
Axelsson, A ;
Elmgren, K ;
Johansson, C .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT, 2003, 508 (03) :542-553
[22]   Measurements of radioxenon in ground level air in South Korea following the claimed nuclear test in North Korea on October 9, 2006 [J].
Ringbom, A. ;
Elmgren, Klas ;
Lindh, Karin ;
Peterson, Jenny ;
Bowyer, Theodore W. ;
Hayes, James C. ;
McIntyre, Justin I. ;
Panisko, Mark ;
Williams, Richard .
JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY, 2009, 282 (03) :773-779
[23]  
Ringbom A., 2007, ANAL RADIOXENON GROU
[24]   A long distance measurement of radioxenon in Yellowknife, Canada, in late October 2006 [J].
Saey, P. R. J. ;
Bean, M. ;
Becker, A. ;
Coyne, J. ;
d'Amours, R. ;
De Geer, L.-E. ;
Hogue, R. ;
Stocki, T. J. ;
Ungar, R. K. ;
Wotawa, G. .
GEOPHYSICAL RESEARCH LETTERS, 2007, 34 (20)
[25]   The influence of radiopharmaceutical isotope production on the global radioxenon background [J].
Saey, Paul R. J. .
JOURNAL OF ENVIRONMENTAL RADIOACTIVITY, 2009, 100 (05) :396-406
[26]   Notes on radioxenon measurements for CTBT verification purposes [J].
Saey, PRJ ;
De Geer, LE .
APPLIED RADIATION AND ISOTOPES, 2005, 63 (5-6) :765-773
[27]  
SAEY PRJ, 2010, PURE APPL GEOPHYS TO, V167
[28]  
SCHOENGOLD CR, 1996, DOENV317 NEV OP OFF
[29]   Automated radioxenon monitoring for the comprehensive nuclear-test-ban treaty in two distinctive locations: Ottawa and Tahiti [J].
Stocki, TJ ;
Blanchard, X ;
D'Amours, R ;
Ungar, RK ;
Fontaine, JP ;
Sohier, M ;
Bean, M ;
Taffary, T ;
Racine, J ;
Tracy, BL ;
Brachet, G ;
Jean, M ;
Meyerhof, D .
JOURNAL OF ENVIRONMENTAL RADIOACTIVITY, 2005, 80 (03) :305-326
[30]   Low level noble gas measurements in the field and laboratory in support of the Comprehensive Nuclear-Test-Ban Treaty [J].
Stocki, TJ ;
Bean, M ;
Ungar, RK ;
Toivonen, H ;
Zhang, WH ;
Whyte, J ;
Meyerhof, D .
APPLIED RADIATION AND ISOTOPES, 2004, 61 (2-3) :231-235