Germanium and Silicon Nanocrystal Thin-Film Field-Effect Transistors from Solution

被引:118
作者
Holman, Zachary C. [1 ]
Liu, Chin-Yi [1 ]
Kortshagen, Uwe R. [1 ]
机构
[1] Univ Minnesota, Dept Mech Engn, Minneapolis, MN 55455 USA
关键词
Nanocrystal; transistor; FET; germanium; silicon; thin film; QUANTUM DOTS; TRANSPORT-PROPERTIES; HYDROGEN; SURFACE; SOLIDS; DESORPTION; SEMICONDUCTORS; TEMPERATURE;
D O I
10.1021/nl101413d
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Germanium and silicon have lagged behind more popular II-VI and IV-VI semiconductor materials in the emerging. field of semiconductor nanocrystal thin film devices We report germanium and silicon nanocrystal field-effect transistors fabricated by synthesizing nanocrystals in a plasma, transferring them into solution, and casting thin films Germanium devices show n-type, ambipolar, or p-type behavior depending on annealing temperature with electron and hole mobilities as large as 0 02 and 0 006 cm(2) V-1 s(-1). respectively Silicon devices exhibit n-type behavior without any postdeposition treatment, but are plagued by poor film morphology
引用
收藏
页码:2661 / 2666
页数:6
相关论文
共 39 条
[21]   REVIEW OF GERMANIUM SURFACE PHENOMENA [J].
KINGSTON, RH .
JOURNAL OF APPLIED PHYSICS, 1956, 27 (02) :101-114
[22]   Modeling of particulate coagulation in low pressure plasmas [J].
Kortshagen, U ;
Bhandarkar, U .
PHYSICAL REVIEW E, 1999, 60 (01) :887-898
[23]   Structural, optical, and electrical properties of PbSe nanocrystal solids treated thermally or with simple amines [J].
Law, Matt ;
Luther, Joseph M. ;
Song, Oing ;
Hughes, Barbara K. ;
Perkins, Craig L. ;
Nozik, Arthur J. .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2008, 130 (18) :5974-5985
[24]   High-mobility nanocrystalline silicon thin-film transistors fabricated by plasma-enhanced chemical vapor deposition [J].
Lee, CH ;
Sazonov, A ;
Nathan, A .
APPLIED PHYSICS LETTERS, 2005, 86 (22) :1-3
[25]   Preparation and characterisation of luminescent alkylated-silicon quantum dots [J].
Lie, LH ;
Duerdin, M ;
Tuite, EM ;
Houlton, A ;
Horrocks, BR .
JOURNAL OF ELECTROANALYTICAL CHEMISTRY, 2002, 538 :183-190
[26]   Hybrid Solar Cells from P3HT and Silicon Nanocrystals [J].
Liu, Chin-Y ;
Holman, Zachary C. ;
Kortshagen, Uwe R. .
NANO LETTERS, 2009, 9 (01) :449-452
[27]   High-yield plasma synthesis of luminescent silicon nanocrystals [J].
Mangolini, L ;
Thimsen, E ;
Kortshagen, U .
NANO LETTERS, 2005, 5 (04) :655-659
[28]   All-inorganic field effect transistors fabricated by printing [J].
Ridley, BA ;
Nivi, B ;
Jacobson, JM .
SCIENCE, 1999, 286 (5440) :746-749
[29]   Coulomb blockade and hopping conduction in PbSe quantum dots [J].
Romero, HE ;
Drndic, M .
PHYSICAL REVIEW LETTERS, 2005, 95 (15)
[30]   Solution-processed silicon films and transistors [J].
Shimoda, T ;
Matsuki, Y ;
Furusawa, M ;
Aoki, T ;
Yudasaka, I ;
Tanaka, H ;
Iwasawa, H ;
Wang, DH ;
Miyasaka, M ;
Takeuchi, Y .
NATURE, 2006, 440 (7085) :783-786