Near-field spectroscopy of silicon dioxide thin films

被引:116
作者
Zhang, L. M. [1 ]
Andreev, G. O. [2 ]
Fei, Z. [2 ]
McLeod, A. S. [2 ]
Dominguez, G. [3 ]
Thiemens, M. [3 ]
Castro-Neto, A. H. [4 ,5 ]
Basov, D. N. [2 ]
Fogler, M. M. [2 ]
机构
[1] Boston Univ, Dept Phys, Boston, MA 02215 USA
[2] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA
[3] Univ Calif San Diego, Dept Chem, La Jolla, CA 92093 USA
[4] Natl Univ Singapore, Graphene Res Ctr, Singapore 117542, Singapore
[5] Natl Univ Singapore, Dept Phys, Singapore 117542, Singapore
关键词
SURFACE-ENHANCED SPECTROSCOPY; ELASTIC LIGHT-SCATTERING; OPTICAL MICROSCOPY; SPHERE; SUBSTRATE; NANOSCOPY; PLASMONS; SCALE; PROBE; TIP;
D O I
10.1103/PhysRevB.85.075419
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We analyze the results of scanning near-field infrared spectroscopy performed on thin films of a-SiO2 on Si substrate. The measured near-field signal exhibits surface-phonon resonances whose strength has a prominent thickness dependence in the range from 2 to 300 nm. These observations are compared with calculations in which the tip of the near-field infrared spectrometer is modeled either as a point dipole or an elongated spheroid. The latter model accounts for the antenna effect of the tip and gives a better agreement with the experiment. Possible applications of the near-field technique for depth profiling of layered nanostructures are discussed.
引用
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页数:8
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