共 28 条
Investigation of non-halogenated solvent mixtures for high throughput fabrication of polymer-fullerene solar cells
被引:68
作者:

Schmidt-Hansberg, Benjamin
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机构:
Karlsruhe Inst Technol KIT, Inst Thermal Proc Engn, D-76131 Karlsruhe, Germany Karlsruhe Inst Technol KIT, Inst Thermal Proc Engn, D-76131 Karlsruhe, Germany

Sanyal, Monamie
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机构:
Max Planck Inst Met Res, D-70569 Stuttgart, Germany Karlsruhe Inst Technol KIT, Inst Thermal Proc Engn, D-76131 Karlsruhe, Germany

Grossiord, Nadia
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机构:
Holst Ctr TNO, NL-5605 KN Eindhoven, Netherlands Karlsruhe Inst Technol KIT, Inst Thermal Proc Engn, D-76131 Karlsruhe, Germany

Galagan, Yulia
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Holst Ctr TNO, NL-5605 KN Eindhoven, Netherlands Karlsruhe Inst Technol KIT, Inst Thermal Proc Engn, D-76131 Karlsruhe, Germany

Baunach, Michael
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Karlsruhe Inst Technol KIT, Inst Thermal Proc Engn, D-76131 Karlsruhe, Germany Karlsruhe Inst Technol KIT, Inst Thermal Proc Engn, D-76131 Karlsruhe, Germany

Klein, Michael F. G.
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机构:
Karlsruhe Inst Technol KIT, Light Technol Inst, D-76131 Karlsruhe, Germany Karlsruhe Inst Technol KIT, Inst Thermal Proc Engn, D-76131 Karlsruhe, Germany

Colsmann, Alexander
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机构:
Karlsruhe Inst Technol KIT, Light Technol Inst, D-76131 Karlsruhe, Germany Karlsruhe Inst Technol KIT, Inst Thermal Proc Engn, D-76131 Karlsruhe, Germany

Scharfer, Philip
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Karlsruhe Inst Technol KIT, Inst Thermal Proc Engn, D-76131 Karlsruhe, Germany Karlsruhe Inst Technol KIT, Inst Thermal Proc Engn, D-76131 Karlsruhe, Germany

Lemmer, Uli
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h-index: 0
机构:
Karlsruhe Inst Technol KIT, Light Technol Inst, D-76131 Karlsruhe, Germany Karlsruhe Inst Technol KIT, Inst Thermal Proc Engn, D-76131 Karlsruhe, Germany

Dosch, Helmut
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DESY, D-22607 Hamburg, Germany Karlsruhe Inst Technol KIT, Inst Thermal Proc Engn, D-76131 Karlsruhe, Germany

Michels, Jasper
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h-index: 0
机构:
Holst Ctr TNO, NL-5605 KN Eindhoven, Netherlands Karlsruhe Inst Technol KIT, Inst Thermal Proc Engn, D-76131 Karlsruhe, Germany

Barrena, Esther
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h-index: 0
机构:
Max Planck Inst Met Res, D-70569 Stuttgart, Germany
CSIC, ICMAB, Bellaterra 08193, Spain Karlsruhe Inst Technol KIT, Inst Thermal Proc Engn, D-76131 Karlsruhe, Germany

Schabel, Wilhelm
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h-index: 0
机构:
Karlsruhe Inst Technol KIT, Inst Thermal Proc Engn, D-76131 Karlsruhe, Germany Karlsruhe Inst Technol KIT, Inst Thermal Proc Engn, D-76131 Karlsruhe, Germany
机构:
[1] Karlsruhe Inst Technol KIT, Inst Thermal Proc Engn, D-76131 Karlsruhe, Germany
[2] Max Planck Inst Met Res, D-70569 Stuttgart, Germany
[3] Holst Ctr TNO, NL-5605 KN Eindhoven, Netherlands
[4] Karlsruhe Inst Technol KIT, Light Technol Inst, D-76131 Karlsruhe, Germany
[5] DESY, D-22607 Hamburg, Germany
[6] CSIC, ICMAB, Bellaterra 08193, Spain
关键词:
Organic photovoltaic;
Drying process;
P3HT:PCBM;
Morphology;
Grazing incidence X-ray diffraction (GIXD);
Knife coating;
MORPHOLOGY;
MOBILITY;
D O I:
10.1016/j.solmat.2011.09.059
中图分类号:
TE [石油、天然气工业];
TK [能源与动力工程];
学科分类号:
0807 ;
0820 ;
摘要:
The rapidly increasing power conversion efficiencies of organic solar cells are an important prerequisite towards low cost photovoltaic fabricated in high throughput. In this work we suggest indane as a non-halogenated replacement for the commonly used halogenated solvent o-dichlorobenzene. Indane was blended with the higher volatile solvents chloroform or toluene or o-xylene in order to improve wettability and to reduce drying time. The combination of high volatile solvents with the less volatile host solvent indane allows for an increased fabrication speed due to a reduction of the overall drying time and provides films with good light absorption behavior and high polymer crystallinity. For the solvent mixture toluene-indane, solar cell performance is comparable to the o-dichlorobenzene reference device indicating this mixture as a suitable replacement for increased productivity without drawbacks in nanomorphology as investigated by atomic force microscopy (AFM) and grazing incidence X-ray diffraction (GIXD). This study provides a fundamental understanding on solvent mixture drying kinetics and can aid the ink formulation. (C) 2011 Elsevier B.V. All rights reserved.
引用
收藏
页码:195 / 201
页数:7
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Max Planck Inst Met Res, D-70569 Stuttgart, Germany Karlsruhe Inst Technol, Light Technol Inst, D-76131 Karlsruhe, Germany

Klein, Michael F. G.
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Karlsruhe Inst Technol, Light Technol Inst, D-76131 Karlsruhe, Germany Karlsruhe Inst Technol, Light Technol Inst, D-76131 Karlsruhe, Germany

Pfaff, Marina
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Karlsruhe Inst Technol, Electron Microscopy Lab, D-76131 Karlsruhe, Germany
Karlsruhe Inst Technol, CFN, D-76131 Karlsruhe, Germany Karlsruhe Inst Technol, Light Technol Inst, D-76131 Karlsruhe, Germany

Schnabel, Natalie
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机构: Karlsruhe Inst Technol, Light Technol Inst, D-76131 Karlsruhe, Germany

Jaiser, Stefan
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机构: Karlsruhe Inst Technol, Light Technol Inst, D-76131 Karlsruhe, Germany

Vorobiev, Alexei
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机构:
European Synchrotron Radiat Facil, F-38043 Grenoble 9, France Karlsruhe Inst Technol, Light Technol Inst, D-76131 Karlsruhe, Germany

Mueller, Erich
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Karlsruhe Inst Technol, Electron Microscopy Lab, D-76131 Karlsruhe, Germany
Karlsruhe Inst Technol, CFN, D-76131 Karlsruhe, Germany Karlsruhe Inst Technol, Light Technol Inst, D-76131 Karlsruhe, Germany

Colsmann, Alexander
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Karlsruhe Inst Technol, Light Technol Inst, D-76131 Karlsruhe, Germany Karlsruhe Inst Technol, Light Technol Inst, D-76131 Karlsruhe, Germany

Scharfer, Philip
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机构: Karlsruhe Inst Technol, Light Technol Inst, D-76131 Karlsruhe, Germany

Gerthsen, Dagmar
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Karlsruhe Inst Technol, Electron Microscopy Lab, D-76131 Karlsruhe, Germany
Karlsruhe Inst Technol, CFN, D-76131 Karlsruhe, Germany Karlsruhe Inst Technol, Light Technol Inst, D-76131 Karlsruhe, Germany

Lemmer, Uli
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Karlsruhe Inst Technol, Light Technol Inst, D-76131 Karlsruhe, Germany Karlsruhe Inst Technol, Light Technol Inst, D-76131 Karlsruhe, Germany

Barrena, Esther
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机构:
Max Planck Inst Met Res, D-70569 Stuttgart, Germany
CSIC, ICMAB, Bellaterra 08193, Spain Karlsruhe Inst Technol, Light Technol Inst, D-76131 Karlsruhe, Germany

Schabel, Wilhelm
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机构: Karlsruhe Inst Technol, Light Technol Inst, D-76131 Karlsruhe, Germany