Effect of layer thickness on the luminescence properties of ZnS/CdS/ZnS quantum dot quantum well

被引:37
作者
Cao, LX [1 ]
Huang, SH
Lü, SZ
Lin, JL
机构
[1] Ocean Univ China, Inst Mat Sci & Engn, Qingdao 266003, Peoples R China
[2] Chinese Acad Sci, Lab Excited State Proc, Changchun 130021, Peoples R China
[3] Chinese Acad Sci, Changchun Inst Opt Fine Mech & Phys, Changchun 130021, Peoples R China
关键词
quantum dot quantum well; ZnS; CdS;
D O I
10.1016/j.jcis.2004.10.066
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
ZnS/CdS/ZnS quantum dot quantum well was prepared. The optical properties of ZnS/CdS/ZnS QDQW with different thickness of US well and ZnS shell were studied, Absorption spectra, emission spectra, and luminescence lifetimes were measured. The observed luminescence was assigned to the bulk donor-acceptor pair recombination of CdS and can be enhanced by increasing the thickness of the CdS well or coating an appropriate thickness of ZnS shell on the surface of the US well. The luminescence enhancement was caused by the relative reduce in the surface effect. The luminescence lifetimes were influenced strongly by the surface state. (c) 2005 Elsevier Inc. All rights reserved.
引用
收藏
页码:516 / 520
页数:5
相关论文
共 27 条
[1]   QUANTUM CRYSTALLITES AND NONLINEAR OPTICS [J].
BRUS, L .
APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING, 1991, 53 (06) :465-474
[2]   ZnS/CdS/ZnS quantum dot quantum well produced in inverted micelles [J].
Cao, LX ;
Huang, SH ;
Shulin, E .
JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2004, 273 (02) :478-482
[3]   LUMINESCENCE AND PHOTOPHYSICS OF CDS SEMICONDUCTOR CLUSTERS - THE NATURE OF THE EMITTING ELECTRONIC STATE [J].
CHESTNOY, N ;
HARRIS, TD ;
HULL, R ;
BRUS, LE .
JOURNAL OF PHYSICAL CHEMISTRY, 1986, 90 (15) :3393-3399
[4]   (CdSe)ZnS core-shell quantum dots: Synthesis and characterization of a size series of highly luminescent nanocrystallites [J].
Dabbousi, BO ;
RodriguezViejo, J ;
Mikulec, FV ;
Heine, JR ;
Mattoussi, H ;
Ober, R ;
Jensen, KF ;
Bawendi, MG .
JOURNAL OF PHYSICAL CHEMISTRY B, 1997, 101 (46) :9463-9475
[5]   A QUANTUM-DOT QUANTUM-WELL - CDS/HGS/CDS [J].
EYCHMULLER, A ;
MEWS, A ;
WELLER, H .
CHEMICAL PHYSICS LETTERS, 1993, 208 (1-2) :59-62
[6]  
HASSELBARTH A, 1993, J PHYS CHEM-US, V97, P5333
[7]   A LIQUID-SOLUTION-PHASE SYNTHESIS OF CRYSTALLINE SILICON [J].
HEATH, JR .
SCIENCE, 1992, 258 (5085) :1131-1133
[8]   Picosecond electronic relaxation in CdS/HgS/CdS quantum dot quantum well semiconductor nanoparticles [J].
Kamalov, VF ;
Little, R ;
Logunov, SL ;
ElSayed, MA .
JOURNAL OF PHYSICAL CHEMISTRY, 1996, 100 (16) :6381-6384
[9]   NANOMETER-SIZED COLLOIDAL GERMANIUM PARTICLES - WET-CHEMICAL SYNTHESIS, LASER-INDUCED CRYSTALLIZATION AND PARTICLE GROWTH [J].
KORNOWSKI, A ;
GIERSIG, M ;
VOGEL, R ;
CHEMSEDDINE, A ;
WELLER, H .
ADVANCED MATERIALS, 1993, 5 (09) :634-636
[10]   Visible photoluminescence from self-assembled InAs quantum dots embedded in AlAs cladding layers [J].
Lee, UH ;
Lee, D ;
Lee, HG ;
Noh, SK ;
Leem, JY ;
Lee, HJ .
APPLIED PHYSICS LETTERS, 1999, 74 (11) :1597-1599