Electrolyte Gate-Controlled Kondo Effect in SrTiO3

被引:156
作者
Lee, Menyoung [1 ]
Williams, J. R. [1 ]
Zhang, Sipei [2 ]
Frisbie, C. Daniel [2 ]
Goldhaber-Gordon, D. [1 ]
机构
[1] Stanford Univ, Dept Phys, Stanford, CA 94305 USA
[2] Univ Minnesota, Dept Chem Engn & Mat Sci, Minneapolis, MN 55455 USA
基金
美国国家科学基金会;
关键词
THIN-FILM TRANSISTORS; INTERFACES; SUPERCONDUCTIVITY; ELECTRONICS; ALLOYS; MAGNETORESISTIVITY; COEXISTENCE; SURFACE; FIELD;
D O I
10.1103/PhysRevLett.107.256601
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We report low-temperature, high-field magnetotransport measurements of SrTiO3 gated by an ionic gel electrolyte. A saturating resistance upturn and negative magnetoresistance that signal the emergence of the Kondo effect appear for higher applied gate voltages. This observation, enabled by the wide tunability of the ionic gel-applied electric field, promotes the interpretation of the electric field-effect-induced 2D electron system in SrTiO3 as an admixture of magnetic Ti3+ ions, i.e., localized and unpaired electrons, and delocalized electrons that partially fill the Ti 3d conduction band.
引用
收藏
页数:5
相关论文
共 41 条
[31]   Origin of the Two-Dimensional Electron Gas Carrier Density at the LaAlO3 on SrTiO3 Interface [J].
Popovic, Zoran S. ;
Satpathy, Sashi ;
Martin, Richard M. .
PHYSICAL REVIEW LETTERS, 2008, 101 (25)
[32]   Highly conductive nanolayers on strontium titanate produced by preferential ion-beam etching [J].
Reagor, DW ;
Butko, VY .
NATURE MATERIALS, 2005, 4 (08) :593-596
[33]   Orbital Reconstruction and the Two-Dimensional Electron Gas at the LaAlO3/SrTiO3 Interface [J].
Salluzzo, M. ;
Cezar, J. C. ;
Brookes, N. B. ;
Bisogni, V. ;
De Luca, G. M. ;
Richter, C. ;
Thiel, S. ;
Mannhart, J. ;
Huijben, M. ;
Brinkman, A. ;
Rijnders, G. ;
Ghiringhelli, G. .
PHYSICAL REVIEW LETTERS, 2009, 102 (16)
[34]   Two-dimensional electron gas with universal subbands at the surface of SrTiO3 [J].
Santander-Syro, A. F. ;
Copie, O. ;
Kondo, T. ;
Fortuna, F. ;
Pailhes, S. ;
Weht, R. ;
Qiu, X. G. ;
Bertran, F. ;
Nicolaou, A. ;
Taleb-Ibrahimi, A. ;
Le Fevre, P. ;
Herranz, G. ;
Bibes, M. ;
Reyren, N. ;
Apertet, Y. ;
Lecoeur, P. ;
Barthelemy, A. ;
Rozenberg, M. J. .
NATURE, 2011, 469 (7329) :189-193
[35]   OXIDE ELECTRONICS Interface takes charge over Si [J].
Schlom, Darrell G. ;
Mannhart, Jochen .
NATURE MATERIALS, 2011, 10 (03) :168-169
[36]   Origin of charge density at LaAlO3 on SrTiO3 heterointerfaces:: Possibility of intrinsic doping [J].
Siemons, Wolter ;
Koster, Gertjan ;
Yamamoto, Hideki ;
Harrison, Walter A. ;
Lucovsky, Gerald ;
Geballe, Theodore H. ;
Blank, Dave H. A. ;
Beasley, Malcolm R. .
PHYSICAL REVIEW LETTERS, 2007, 98 (19)
[37]  
Son J, 2010, NAT MATER, V9, P482, DOI [10.1038/nmat2750, 10.1038/NMAT2750]
[38]   An Emergent Change of Phase for Electronics [J].
Takagi, Hidenori ;
Hwang, Harold Y. .
SCIENCE, 2010, 327 (5973) :1601-1602
[39]   Tunable quasi-two-dimensional electron gases in oxide heterostructures [J].
Thiel, S. ;
Hammerl, G. ;
Schmehl, A. ;
Schneider, C. W. ;
Mannhart, J. .
SCIENCE, 2006, 313 (5795) :1942-1945
[40]   Electric-field-induced superconductivity in an insulator [J].
Ueno, K. ;
Nakamura, S. ;
Shimotani, H. ;
Ohtomo, A. ;
Kimura, N. ;
Nojima, T. ;
Aoki, H. ;
Iwasa, Y. ;
Kawasaki, M. .
NATURE MATERIALS, 2008, 7 (11) :855-858