Self-Assembly and Traveling Wave Ion Mobility Mass Spectrometry Analysis of Hexacadmium Macrocycles

被引:132
作者
Chan, Yi-Tsu [1 ]
Li, Xiaopeng [2 ]
Soler, Monica [1 ]
Wang, Jin-Liang [1 ]
Wesdemiotis, Chrys [1 ,2 ]
Newkome, George R. [1 ,2 ]
机构
[1] Univ Akron, Dept Polymer Sci, Akron, OH 44325 USA
[2] Univ Akron, Dept Chem, Akron, OH 44325 USA
基金
美国国家科学基金会;
关键词
GAS-PHASE; HEXAMERIC METALLOMACROCYCLES; COMPLEXES; CHEMISTRY; ARCHITECTURES; CONSTRUCTION; PRINCIPLE; POLYMERS; STEPWISE;
D O I
10.1021/ja907262c
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Self-assembly of 1,3-di(4'-terpyridinyl)arenes by using the labile tpy-Cd(II)-tpy (where tpy = 2,2':6',2 ''-terpyridine) connectivity afforded access to hexacadmium macrocycles in high yield. These supramolecular assemblies were characterized by traveling wave ion mobility mass spectrometry (TWIM-MS).
引用
收藏
页码:16395 / +
页数:4
相关论文
共 46 条
[1]   Structural investigation of encapsulated fluoride in polyhedral oligomeric silsesquioxane cages using ion mobility mass spectrometry and molecular mechanics [J].
Anderson, Stanley E. ;
Bodzin, Dena J. ;
Haddad, Timothy S. ;
Boatz, Jerry A. ;
Mabry, Joseph M. ;
Mitchell, Connie ;
Bowers, Michael T. .
CHEMISTRY OF MATERIALS, 2008, 20 (13) :4299-4309
[2]   Biomolecule Analysis by Ion Mobility Spectrometry [J].
Bohrer, Brian C. ;
Mererbloom, Samuel I. ;
Koeniger, Stormy L. ;
Hilderbrand, Amy E. ;
Clemmer, David E. .
ANNUAL REVIEW OF ANALYTICAL CHEMISTRY, 2008, 1 (01) :293-327
[3]   GAS-PHASE ION CHROMATOGRAPHY - TRANSITION-METAL STATE SELECTION AND CARBON CLUSTER FORMATION [J].
BOWERS, MT ;
KEMPER, PR ;
VON HELDEN, G ;
VANKOPPEN, PAM .
SCIENCE, 1993, 260 (5113) :1446-1451
[4]   Efficient synthesis of pyridines via a sequential solventless aldol condensation and Michael addition [J].
Cave, GWV ;
Raston, CL .
JOURNAL OF THE CHEMICAL SOCIETY-PERKIN TRANSACTIONS 1, 2001, (24) :3258-3264
[5]  
Clemmer DE, 1997, J MASS SPECTROM, V32, P577
[6]   Expanded ligands - An assembly principle for supramolecular chemistry [J].
Constable, Edwin C. .
COORDINATION CHEMISTRY REVIEWS, 2008, 252 (8-9) :842-855
[7]   Reactivity of self-assembled supramolecular complexes in the gas phase: A supramolecular neighbor group effect [J].
Engeser, Marianne ;
Rang, Alexander ;
Ferrer, Montserrat ;
Gutierrez, Albert ;
Baytekin, H. Tarik ;
Schalley, Christoph A. .
INTERNATIONAL JOURNAL OF MASS SPECTROMETRY, 2006, 255 :185-194
[8]   Biomolecular structural separations by ion mobility-mass spectrometry [J].
Fenn, Larissa S. ;
McLean, John A. .
ANALYTICAL AND BIOANALYTICAL CHEMISTRY, 2008, 391 (03) :905-909
[9]   Coordination assemblies from a Pd(II)-cornered square complex [J].
Fujita, M ;
Tominaga, M ;
Hori, A ;
Therrien, B .
ACCOUNTS OF CHEMICAL RESEARCH, 2005, 38 (04) :369-378
[10]   Construction of Multifunctional Cuboctahedra via Coordination-Driven Self-Assembly [J].
Ghosh, Koushik ;
Hu, Jiming ;
White, Henry S. ;
Stang, Peter J. .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2009, 131 (19) :6695-+