Infrared imaging of single nanoparticles via strong field enhancement in a scanning nanogap

被引:87
作者
Cvitkovic, A. [1 ]
Ocelic, N.
Aizpurua, J.
Guckenberger, R.
Hillenbrand, R.
机构
[1] Max Planck Inst Biochem, Nano Photon Grp, D-82152 Martinsried, Germany
[2] Max Planck Inst Biochem, Abt Mol Strukturbiol, D-82152 Martinsried, Germany
[3] Donostia Int Phys Ctr, San Sebastian 20018, Spain
关键词
D O I
10.1103/PhysRevLett.97.060801
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We demonstrate nanoscale resolved infrared imaging of single nanoparticles employing near-field coupling in the nanoscopic gap between the metal tip of a scattering-type near-field optical microscope and the substrate supporting the particles. Experimental and theoretical evidence is provided that highly reflecting or polariton-resonant substrates strongly enhance the near-field optical particle contrast. Using Si substrates we succeeded in detecting Au particles as small as 8 nm (<lambda/1000) at midinfrared wavelengths of about lambda=10 mu m. Our results open the door to infrared spectroscopy of individual nanoparticles, nanocrystals, or macromolecules.
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页数:4
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