Atomic-Resolution Imaging with a Sub-50-pm Electron Probe

被引:355
作者
Erni, Rolf [1 ]
Rossell, Marta D. [1 ]
Kisielowski, Christian [1 ]
Dahmen, Ulrich [1 ]
机构
[1] Lawrence Berkeley Natl Lab, Natl Ctr Electron Microscopy, Berkeley, CA 94720 USA
关键词
MICROSCOPE; CORRECTOR; STEM;
D O I
10.1103/PhysRevLett.102.096101
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Using a highly coherent focused electron probe in a fifth-order aberration-corrected transmission electron microscope, we report on resolving a crystal spacing less than 50 pm. Based on the geometrical source size and residual coherent and incoherent axial lens aberrations, an electron probe is calculated, which is theoretically capable of resolving an ideal 47 pm spacing with 29% contrast. Our experimental data show the 47 pm spacing of a Ge < 114 > crystal imaged with 11%-18% contrast at a 60%-95% confidence level, providing the first direct evidence for sub-50-pm resolution in annular dark-field scanning transmission electron microscopy imaging.
引用
收藏
页数:4
相关论文
共 18 条
[1]   Sub-angstrom resolution using aberration corrected electron optics [J].
Batson, PE ;
Dellby, N ;
Krivanek, OL .
NATURE, 2002, 418 (6898) :617-620
[2]  
Born M., 2003, PRINCIPLES OPTICS
[3]   IMAGE CONTRAST IN A TRANSMISSION SCANNING ELECTRON MICROSCOPE [J].
COWLEY, JM .
APPLIED PHYSICS LETTERS, 1969, 15 (02) :58-&
[4]   Method to measure spatial coherence of subangstrom electron beams [J].
Dwyer, Christian ;
Erni, Rolf ;
Etheridge, Joanne .
APPLIED PHYSICS LETTERS, 2008, 93 (02)
[5]   The S-state model: a work horse for HRTEM [J].
Geuens, P ;
Van Dyck, D .
ULTRAMICROSCOPY, 2002, 93 (3-4) :179-198
[6]   Upper limits for the residual aberrations of a high-resolution aberration-corrected STEM [J].
Haider, M ;
Uhlemann, S ;
Zach, J .
ULTRAMICROSCOPY, 2000, 81 (3-4) :163-175
[7]   Electron microscopy image enhanced [J].
Haider, M ;
Uhlemann, S ;
Schwan, E ;
Rose, H ;
Kabius, B ;
Urban, K .
NATURE, 1998, 392 (6678) :768-769
[8]   3-D reconstruction of the atomic positions in a simulated gold nanocrystal based on discrete tomography: Prospects of atomic resolution electron tomography [J].
Jinschek, J. R. ;
Batenburg, K. J. ;
Calderon, H. A. ;
Kilaas, R. ;
Radmilovic, V. ;
Kisielowski, C. .
ULTRAMICROSCOPY, 2008, 108 (06) :589-604
[9]   SIMULATION OF ANNULAR DARK FIELD STEM IMAGES USING A MODIFIED MULTISLICE METHOD [J].
KIRKLAND, EJ ;
LOANE, RF ;
SILCOX, J .
ULTRAMICROSCOPY, 1987, 23 (01) :77-96
[10]   Detection of single atoms and buried defects in three dimensions by aberration-corrected electron microscope with 0.5-Å information limit [J].
Kisielowski, C. ;
Freitag, B. ;
Bischoff, M. ;
van Lin, H. ;
Lazar, S. ;
Knippels, G. ;
Tiemeijer, P. ;
van der Stam, M. ;
von Harrach, S. ;
Stekelenburg, M. ;
Haider, M. ;
Uhlemann, S. ;
Mueller, H. ;
Hartel, P. ;
Kabius, B. ;
Miller, D. ;
Petrov, I. ;
Olson, E. A. ;
Donchev, T. ;
Kenik, E. A. ;
Lupini, A. R. ;
Bentley, J. ;
Pennycook, S. J. ;
Anderson, I. M. ;
Minor, A. M. ;
Schmid, A. K. ;
Duden, T. ;
Radmilovic, V. ;
Ramasse, Q. M. ;
Watanabe, M. ;
Erni, R. ;
Stach, E. A. ;
Denes, P. ;
Dahmen, U. .
MICROSCOPY AND MICROANALYSIS, 2008, 14 (05) :469-477